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ting phase at the inlet face is considered. The resulting scaling equations incorporate all factors that influence the process and are found in terms of the Darcy number (Da) and
capillary number, (Ca). The proposed scaling equations are
validated against the published experimental data from the
literature.
Introduction
Spontaneous imbibition of an aqueous phase (i.e., the wetting phase, WP) into matrix blocks arising from capillary
forces is an important mechanism to displace the nonwetting
phase (NWP) from fractured reservoirs.[1] This can be either
countercurrent or cocurrent displacement. In countercurrent
spontaneous imbibition (COUCSI) all the permeable faces
of a rock saturated with NWP are brought into contact with
a WP and the WP flows in the opposite direction to the expelled NWP.[2, 3] However, in cocurrent spontaneous imbibition (COCSI) only a portion of the permeable surfaces is in
contact with a WP and, while keeping the remaining permeable surfaces covered by the NWP, both phases flow in the
same direction.
In a typical COCSI experiment, matrix surfaces covered
by WP and NWP are kept constant during the process.[414] In
this case, level of the WP in the fracture system is kept constant at a certain level and there is no viscous force in the
fracture system. We use the same COCSI case in this study.
There are also other cases in which the recovery performance of a matrix block or a stack of matrix blocks under
advancing WP level in the fracture system are studied.[1520]
Despite the fact that the COCSI can take place in fractured reservoir,[19, 21, 22] most attention has been received on
scale-up of COUCSI.[2325] Use of the scaled-up results of
COUCSI experiments leads to pessimistic forecasts regarding
the rate of recovery and final recovery.[10, 18, 26] It has been emphasized that COCSI is more efficient in terms of both final
recovery and displacement rate than COUCSI.[7, 911, 1820, 26, 27]
Due to the significant differences between the recovery performances in these processes, the corresponding scaling
equations cannot interchangeably be used. Several studies
show that the scaling equations developed for the COUCSI
process fail to scale up the COCSI data.[8, 10, 2830]
A few scaling equations have been proposed for recovery
prediction of COCSI.[3133] They have been applied to one-dimensional displacement as no characteristic length has been
defined for the COCSI. These scaling equations do not incor-
166
porate all of the factors influencing the process; consequently, they cannot properly describe the process. The scaling
equation proposed by Rapoport[31] was developed by using
the inspectional analysis of the main governing equations,
making some simplifying assumptions; including that the
prototype WP/NWP viscosity ratio must be duplicated in the
model tests, initial fluid saturations in the prototype must be
duplicated in the model tests, the relative permeability functions must be the same for both the model and the prototype, and the capillary pressure functions for the both the
model and the prototype must be related by direct proportionality. Several studies have attempted to develop the scaling equation of Rapoport (e.g., Ref. [34, 35]) to COUCSI
data only. The scaling equations of Li[32] and Bourbiaux[33]
were derived based on a restricting approximate solution to
the main governing equations. They take the assumption of
piston-like displacement which is valid only for a few particular cases. However, according to Mirzaei-Paiaman and
Masihi,[25] the development of these two scaling equations is
not consistent with common scaling practices.
The main purpose of this study is to present universal scaling equations for one-dimensional COCSI based on the
recent finding of Schmid[36] who notices that the analytical
solution to unidirectional displacement given by McWhorter
and Sunada[37] applies to COCSI with no artificial boundary
conditions. We consider the consistency between the development of the new scaling equations and common practices
as was considered for COUCSI in Mirzaei-Paiaman and
Masihi.[25] These new scaling equations are rewritten in terms
[a] Dr. A. Mirzaei-Paiaman, Dr. M. Masihi
Department of Chemical and Petroleum Engineering
Sharif University of Technology
P.O. Box 11365-9465, Azadi Ave., Tehran (Iran)
E-mail: Mirzaei1986@gmail.com
[b] Dr. A. Mirzaei-Paiaman
Department of Petroleum Engineering
NISOC, Ahvaz (Iran)
uw f Sw ut DSw
@Sw
@x
@Sw
@f Sw @
@S
DSw w
ut
@x
@x
@t
@x
f Sw
krw mnw
krw mnw krnw mw
dP
in which kr is the relative permeability, m is the dynamic viscosity, k is the absolute permeability, and Pc is the capillary
pressure.
The appropriate initial and boundary conditions can be defined as,[37]
Sw x; 0 Swi
Sw 1; t Swi
uw 0; t At1=2
ut
in which fi is the WP fraction of the total efflux, R uw 0;t
fn
f fi R
1 fi R
9
R Sw;BC bSw Db
Sw
F bfn b db
F Sw 1 R Sw;BC
Sw Swi DSw
Swi
F Sw fn Sw dSw
10
xSw ; t
2A1 fi R 0
F Sw t1=2
11
12
Z Sw;BC
Sw Swi DSw
dSw
A
21 fi R Swi
F Sw fn Sw
13
Using this equation, Schmid[36] noticed that the inlet boundary condition imposed by McWhorter and Sunada[37] to
solve the original problem is redundant for the case of both
COUCSI and COCSI and the solution given in Equation (11) describes the standard situation found in the laboratory experiments. Schmid and Geiger[23, 24] and Mirzaei-Paiaman and Masihi[25] use this finding to develop the appropriate scaling equations for COUCSI cases. Mirzaei-Paiaman
et al.[38] used the analytical solution for the COUCSI case to
167
McWhorter and Sunada considered a special case of unidirectional displacement that could be realized in laboratory
by using a semipermeable membrane that is permeable to
only the WP (i.e., R = 1). However in practice if a NWP is initially present and is being displaced by a WP, depending on
the magnitude of the forced injection rate, three flow regimes may occur in a linear flow domain.[39, 40] If there is no
forced injection at the inlet boundary, there will be countercurrent flow (with respect to the NWP) at the inlet face implying R < 1 (regime 1). As the injection rate increases up to
some critical value, the region of countercurrent flow continually decreases but the R < 1 condition remains (regime 2).
Countercurrent flow ceases as the injection rate at the inlet
reaches this critical value and R = 1 (regime 3). Unidirectional displacement only occurs if the injection rate equals or exceeds this critical value.[39, 40] In the COCSI case considered
in this study there is no forced injection at the inlet, and
therefore regime 1 is expected to take place. Several studies
confirm the existence of some backflow production of NWP
in the inlet in regime 1.[7, 9, 10, 18] Thus, the solution presented
by McWhorter and Sunada[37] when applied to COCSI
should be slightly modified to account for the backflow production of NWP at the inlet boundary. This can be achieved
by assigning a value not much smaller and not very close to
1 (e.g., 0.95) to R and proceeding with the analytical solution. The reason for the choice of such a value comes from
the experimental observations.[7, 9, 10]
The main obstacle of the iterative approach proposed by
McWhorter and Sunada[37] is that to obtain the Sw,m values
from Sw,BC (in which Sw,m is the WP saturation reached after
forced displacement) and R = 1, difficulties can be encountered for computing the solution integrals, because the
values of F(Sw) and fn(Sw) approach each other. This causes
the iterative process to become unstable.[41] Our strategy to
account for the contribution of the backflow production by
assuming R
6 1 avoids the occurrence of any instability.
As the analytic solution presented by McWhorter and
Sunada[37] can be applied to COCSI with no artificial boundary condition,[36] after consideration of the contribution of
the backflow production, it sufficiently incorporates all the
factors influencing the COCSI process.
168
QW
uw dt 2WAt1=2
14
in which W is the surface area perpendicular to flow direction. Similarly the ultimate cumulative recovery, Q1, defined
as the cumulative recovery of NWP up to the time t* at
which the imbibition front reaches the end of the linear
system L can be derived as:
Q1 W
uw dt 2WAt* 1=2
15
Q1
t*
16
17
t*
L
2AF 0 Swi 1 fi R
2
18
t
Q1
L
19
Q1
Vp
Vi
20
t
Vp L
21
Q
2A
t1=2
Vi L1 Swi
22
tD
23
2A 1=2
t
L
24
q
k
R Swi
dJ
w
f Sw mnw
krnw dSw
Sw;BC F Sw fn Sw
db
30
q
R Swi f Sw mm krnw dSdJ
k
s
Q
Sw;BC F Sw fn Sw db
Vi
L vw mw 1 Swi 1 fi R
31
s
Q
Vp
L vw mw
1 fi R
w
nw
Da
k
L2
32
The generalized capillary number Ca representing the relative effect of viscous forces versus interfacial tension can further be written as:
R Sw;BC Swi Sw f Sw mm krnw dSdJ
dSw
vw mw Swi
F Sw fn Sw
2
s R Sw;BC f Sw mm krnw dSdJ
Swi
F Sw fn Sw dSw
w
nw
CaQ1
nw
tD;Vi
2A
t1=2
L1 Swi
25
CaVp
db
vw mw 1 Swi 1 fi R
s R Swi f Sw mm krnw dSdJ
Sw;BC F Sw fn Sw db
w
nw
Sw;BC F Sw fn Sw
CaVi
33
vw mw
1 f i R
s R Swi f Sw mm krnw dSdJ
nw
34
35
Q
2A2 F 0 Swi 1 fi R
Q1
Luw
26
Equation (20) gives the relationship between the Darcy velocity uw and the linear velocity vw as:
uw
vw
t1=2
F 0 Swi 1 fi R
27
28
Q1
L vw mw R Sw;BC Swi Sw f Sw mm krnw dSdJ
dSw
Swi
F Sw fn Sw
w
nw
nw
29
be rewritten as Ca implying that during COCSI, the recovery is controlled by the Darcy and Capillary numbers.
169
L
k [m2]
[cm]
HV1
HV2
HV3
HV4
BK1
AK1
AK2
ST1
9.7
19.9
49.8
84.8
29
9.5
9.5
5.0
0.35
0.35
0.36
0.36
0.39
0
0
0
1.8 10-15
2 10-15
2 10-15
1.6 10-15
1.37 10-13
7 10-15
7 10-15
2 10-15
mnw
s [mN m1] End End Maximum F(Swi) A [ps]
mw
[mPa s] [mPa s]
point point Pc [kPa]
krw
krnw
0.27
0.28
0.28
0.27
0.23
0.69
0.69
0.43
1
1
1
1
1.2
1
1
1
11.5
11.5
11.5
11.5
1.5
0.0182
0.84
0.95
49
49
49
49
35
72
51.4
46
0.14
0.12
0.10
0.12
0.06
0.09
0.15
0.30
170
0.98
0.97
0.95
0.95
0.47
1.00
1.00
1.00
480.1
461.2
458.5
512.8
12.5
428.6
200.4
541.5
4.7
5.2
5.7
5.4
4.3
1.0
1.6
1.4
9.5 10-6
1.7 10-5
2.0 10-5
1.7 10-5
2.6 10-5
4.8 10-4
4.6 10-5
5.4 10-5
Figure 1. Recovery in terms of different reference volumes: a) ultimate recovery, b) pore volume, and c) initial NWP in place versus time for the experiments collected from the literature.
171
Figure 3. Recovery in terms of different reference volumes: a) ultimate recovery, b) pore volume, and c) initial NWP in place versus the scaling equation
of Ma et al.[34]
172
Figure 4. Recovery in terms of different reference volumes: a) ultimate recovery, b) pore volume, and c) initial NWP in place versus the scaling equation
of Mason et al.[35]
Figure 5. Recovery in terms of different reference volumes: a) ultimate recovery, b) pore volume, and c) initial NWP in place versus the scaling equation
of Li.[32]
Inserting Equations (3), (4), (8), (12), and (28) into the dimensionless time equations brings them into the new forms
as:
v
u q
u2s k
t
1=2
36
t
tD tD;Vp tD;Vi G
mnw L2
in which G, a group of variables, differs (Table 2).
Our objective is to extract a simple scaling equation from
Equation (36). We note that G is a function of wettability, initial wetting phase saturation, fluid viscosity, and pore structure. Therefore the exclusion of G from the scaling equation
r
p !
[Eq. (36)] makes this equation
Energy Technol. 2014, 2, 166 175
2s
k
mnw L2
t1=2
independent
Figure 6. Recovery in terms of different reference volumes: a) ultimate recovery, b) pore volume, and c) initial NWP in place versus the corresponding
new scaling equations.
173
R S f S k dSdJ
dSw
F S f S
S
G q
R S S S f S k dSdJ
w
w;BC
wi
w;BC
wi
rnw
F Sw fn Sw
Swi
dSw
s
R S S S f S k dSdJ
tD;Vp
w;BC
wi
rnw
F Sw fn Sw
1fi R2
Swi
dSw
s
R S S S f S k dSdJ
tD;Vi
w;BC
tD;simplified
rnw
v
q
u
k
u
2s
t
1=2
p 2 t
mnw mw mnw L
Swi
wi
rnw
F Sw fn Sw
1Swi 2 1fi R2
dSw
37
Conclusions
The following conclusions can be drawn from this work:
* As the analytical solution to unidirectional displacement
given by McWhorter and Sunada[37] applies to COCSI,[36]
suitable scaling equations for one-dimensional COCSI can
be found by using this solution.
* Backflow production of the NWP at the inlet open boundary is inherent to COCSI and its contribution to the process should be taken into account when using the analytical solution given by McWhorter and Sunada[37] and when
presenting new scaling equations.
* The strategy to account for the contribution of the backflow production by assuming R
6 1 avoids the occurrence
of the possible instabilities in computing the integrals in
the McWhorter and Sunada[37] solution.
* The new scaling equations presented in this study are universal, incorporating all factors influencing the process, as
174
Figure 7. Recovery in terms of different reference volumes: a) ultimate recovery, b) pore volume, and c) initial NWP in place versus the new simplified
scaling equation.
Acknowledgements
The authors thank Sharif University of Technology and the
Research and Technology Departments of NIOC and NISOC
for permission to publish this paper.
[20] H. Karimaie, O. Torster, J. Pet. Sci. Eng. 2007, 58, 293 308.
[21] A. Firoozabadi, J. Can. Pet. Technol. 2000, 39, 13 17.
[22] F. H. Qasem, I. S. Nashawi, R. G. Muhammad, I. Mir, J. Pet. Sci. Eng.
2008, 60, 39 50.
[23] K. S. Schmid, S. Geiger, Water Resour. Res. 2012, 48, http://
dx.doi.org/10.1029/2011WR011566.
[24] K. S. Schmid, S. Geiger, J. Pet. Sci. Eng. 2013, 101, 44 61.
[25] A. Mirzaei-Paiaman, M. Masihi, Energy Fuels 2013, 27, 4662 4676.
[26] D. Zhou, L. Jia, J. Kamath, R. A. Kovscek, J. Pet. Sci. Eng. 2002, 33,
61 74.
[27] E. R. Rangel-German, R. A. Kovscek, J. Pet. Sci. Eng. 2002, 36, 45
60.
[28] A. Kantzas, M. Pow, K. Allsopp, D. Marentette, Paper no. 97 181,
Seventh Petroleum Conference of the South Saskatchewan Section,
The Petroleum Society of CIM, Regina, October, 19 22, 1997.
[29] K. Li, K. Chow, R. N. Horne, SPE Western Regional/AAPG Pacific
Section Joint Meeting, 20 22 May Anchorage, Alaska, 2002,
DOI:10.2118/76727-MS.
[30] C. U. Hatiboglu, T. Babadagli, J. Pet. Sci. Eng. 2010, 70, 214 228.
[31] L. A. Rapoport, Trans. AIME 1955, 204, 143 150.
[32] K. Li, J. Contam. Hydrol. 2007, 89, 218 230.
[33] B. Bourbiaux, International Petroleum Technology Conference, 7 9
December, Doha, Qatar, 2009, DOI:10.2523/13909-MS.
[34] S. Ma, X. Zhang, N. R. Morrow, Annual Technical Meeting of Petroleum Society of Canada, Jun 7 9, Calgary, Alberta, 1955,
DOI:10.2118/95-94.
[35] G. Mason, H. Fischer, N. R. Morrow, D. W. Ruth, J. Pet. Sci. Eng.
2010, 72, 195 205.
[36] K. S. Schmid, PhD thesis, Institute of Petroleum Engineering, HeriotWatt University, 2012, Available online at http://www.ros.hw.ac.uk/
bitstream/10399/2547/1/SchmidKS_0312_pe.pdf.
[37] D. B. McWhorter, D. K. Sunada, Water Resour. Res. 1990, 26, 399
413.
[38] A. Mirzaei-Paiaman, M. Masihi, D. C. Standnes, Energy Fuels 2013,
27, 7360 7368.
[39] Z.-X. Chen, G. S. Bodvarsson, P. A. Witherspoon, Water Resour. Res.
1992, 28, 1477 1478.
[40] Z.-X. Chen, G. S. Bodvarsson, P. A. Witherspoon, SPE Annual Technical Conference and Exhibition, 23 26 September, New Orleans,
Louisiana, 1990, 10.2118/20517-MS.
[41] R. Fuck, J. Mikyska, M. Benes, T. H. Illangasekare, Vadose Zone J.
2007, 6, 93 104.
[42] J. Bear, Dynamics of Fluids in Porous Media, Dover, New York,
1972.
[43] B. Zappoli, R. Cherrier, D. Lasseux, J. Ouazzani, Y. Garrabos,
arxiv.org/abs/cond-mat/0601196 [cond-mat.stat-mech], 2006.
[44] A. Graue, T. Bognoe, R. Moe, B. Baldwin, E. A. Spinler, D. Maloney,
SCA paper 9907, International Symposium of the Society of Core Analysts, 1999.
[45] J. M. Schembre, A. R. Kovscek, Transp. Porous Media 2006, 65, 31
51.
[46] M. A. Fern, A. Haugen, S. Wickramathilaka, J. Howard, A. Graue,
G. Mason, N. R. Morrow, J. Pet. Sci. Eng. 2013, 101, 1 11.
[47] X. M. Zhou, N. R. Morrow, S. X. Ma, SPE J. 2000, 5, 199 207.
[48] X. Xie, N. R. Morrow, Proceedings of the International Symposium of
the Society of Core Analysis Meeting, Abu Dhabi, UAE, October,
2000.
[49] H. Dehghanpour, H. A. Zubair, A. Chhabra, A. Ullah, Energy Fuels
2012, 26, 5750 5758.
[50] H. Dehghanpour, Q. Lan, Y. Saeed, H. Fei, Z. Qi, Energy Fuels 2013,
27, 3039 3049.
175