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Received 20 March 2006; received in revised form 13 December 2006; accepted 18 January 2007
Abstract
Acceleration of premixed laminar flames in the early stages of burning in long tubes is considered. The accel-
eration mechanism was suggested earlier by Clanet and Searby [Combust. Flame 105 (1996) 225]. Acceleration
happens due to the initial ignition geometry at the tube axis when a flame develops to a finger-shaped front, with
surface area growing exponentially in time. Flame surface area grows quite fast but only for a short time. The
analytical theory of flame acceleration is developed, which determines the growth rate, the total acceleration time,
and the maximal increase of the flame surface area. Direct numerical simulations of the process are performed for
the complete set of combustion equations. The simulations results and the theory are in good agreement with the
previous experiments. The numerical simulations also demonstrate flame deceleration, which follows acceleration,
and the so-called tulip flames.
2007 Published by Elsevier Inc. on behalf of The Combustion Institute.
Keywords: Premixed flames; Flame acceleration; Tulip flames; Direct numerical simulations
by the continuity equation and the equation for the flame front
1 v df
(w) + = 0. (4) ( 1) 1 f2 = 1. (13)
d
According to Eq. (13), we can separate two opposite
The boundary condition at the end-wall = 0 is
regimes of flame propagation: when the flame skirt
v = 0. We are interested in the flow along the wall,
is close to the axis f 1, and when it is close to the
in the limit 0. In the fuel mixture (labeled 1)
wall 1f 1. In the limit of f 1, the flame prop-
the flow is potential; we assume
agates with the velocity df /d = (or R f = Uf ).
The same velocity takes place for an expanding hemi-
v1 = A1 , (5)
spherical flame front. In the other case of 1 f
where the factor A1 may depend on time. The as- 1, the flame propagation velocity is df /d = 1 (or
sumption is consistent with the porous piston effect R f = Uf ). In that limit a locally cylindrical flame skirt
as the flame approaches the tube wall. In the hemi- approaches the wall; the radial velocity of the fresh
spherical regime of flame propagation it works only fuel mixture tends to zero, and the flame skirt prop-
sufficiently close to the wall as the leading term in agates with the planar flame velocity with respect to
for 0. Then the radial velocity in the fuel mixture the tube end wall. Integrating Eq. (13) with the initial
is calculated from Eq. (4) as condition f = 0 at = 0, we find
A 1 1 + f
w1 = 1 . (6) = ln , (14)
2 2 f
or
In Eq. (6) we have taken into account the bound-
ary condition at the side-wall of the tube w = 0 at exp(2 ) 1
f = = tanh( ), (15)
= 1. The velocity distribution in the burnt matter exp(2 ) + 1
(labeled 2) takes the form where
v2 = A2 , (7) = ( 1). (16)
A
w2 = 2 . (8) According to Eq. (15), the flame velocity is equal
2 to the velocity of a hemispherical front close to the
In general, the flow in the burnt matter of Fig. 1 is ro- axis, when 2 1 and f = (or Rf = Uf t).
tational because of the curved flame shape. However, Respectively, one should expect transition to the
close to the wall, the flame front is locally cylindri- finger-shape at the characteristic time
cal and the flow (7) and (8) is potentialy similar to (5)
and (6). In Eq. (8) we have also taken into account the sph 1/2, (17)
boundary condition at the tube axis w = 0 at = 0. when the flame skirt is at f 0.46/. Of course,
To complete the solution we consider the matching there is no exact mathematical definition of the tran-
conditions at the flame front = f , sition time. Still, the characteristic time, Eq. (17),
comes as a parameter into Eq. (15) and may be com-
df
w1 = 1, (9) pared to the experiments [20]. For the expansion fac-
d tors = 68, typical for propane flames, we find
w1 w2 = 1, (10) 5.57.5 and 0.06 < sph < 0.09. The theoretical
v1 = v2 . (11) evaluation (17) agrees quite well with the experimen-
tal estimates sph 0.1 [20] taking into account a
The condition (9) specifies the fixed propagation ve- rather vague definition of the value. Transition to the
locity Uf of the flame front with respect to the fuel finger shape takes place approximately when the
mixture (which is unity in scaled variables). The con- flame skirt has moved halfway to the tube side wall. It
ditions (10) and (11) describe the jump of the normal is much easier to determine the time instant when the
velocity and continuity of the tangential velocity at flame skirt touches the tube wall. Substituting f = 1
the front. We stress that Eq. (11) applies only at the into Eq. (14), we obtain
flame skirt close to the wall and it follows from the
irrotational assumption combined with the cylindrical 1 +
wall = ln . (18)
flame shape, i.e., no shear across the flame front. Sub- 2
stituting Eqs. (5)(8) into Eqs. (9)(11), we obtain For the expansion factors = 68 we find 0.23 <
wall < 0.28, which is in very good agreement with
A1 = A2 = 2( 1)f , (12) the experimental evaluation wall 0.26 [20]. Thus,
266 V. Bychkov et al. / Combustion and Flame 150 (2007) 263276
Eqs. (24), (27), and (28) reduce to (ur ) + (uz ur zr )
t z
f = (1 )1/ . (29) 1 2 P 1
+ r ur rr = , (34)
r r r r
We stress that the solution (29) does not satisfy the
boundary condition at the axis f/ = 0 at = 0. + ( + P )uz zz uz zr ur + qz
t z
This is, of course, a consequence of the approxima-
1
tion + r ( + P )ur rr ur zr uz + qr
r r
2
1/2
f f = 0, (35)
1+ (30)
1 Y
(Y ) + rur Y r
t r r Sc r
used in Eq. (25) in the limit of 1 1. Still, the
Y
principal contribution to the flame surface area comes + uz Y
z Sc z
from the flame skirt. Another shortcoming of the eval-
Y
uation (29) is that we adopted the potential flow (7) = exp(Ea /Rp T ), (36)
and (8) everywhere in the burnt matter, while in re- R
ality it holds only close to the tube end wall and to where
the tube axis. Outside of these regions, the flow may
2
be rotational because of the curved flame shape. Us- = (QY + CV T ) + uz + u2r (37)
ing the evaluation (29), the scaled surface area of the 2
curved flame front is calculated as is the total energy per unit volume, Y is the mass frac-
tion of the fuel mixture, Q is the energy release in the
1 2
2 f reaction, and CV is the heat capacity per unit mass
Sw / R = 2 1 + d at constant volume. We consider a single irreversible
0 reaction of the first order. Temperature dependence
1 of the reaction rate obeys the Arrhenius law with the
f 2 activation energy Ea and the constant of time dimen-
2 d = 2 . (31)
+1 sion R . The stress tensor ij is
0
Thus, for stoichiometric propane flames with = 8, 4 uz 2 ur 2 ur
zz = , (38)
we should expect a maximal flame surface area 3 z 3 r 3 r
as large as Sw / R 2 14.2. Of course, order-of- 4 ur 2 uz 2 ur
magnitude evaluations may be obtained within an rr = , (39)
3 r 3 z 3 r
even simpler and cruder approximation of a cylindri-
4 ur 2 uz 2 ur
cal shape of radius R and height R with Sw / R 2 = , (40)
2. Relative difference between this approximation 3 r 3 z 3 r
and Eq. (31) is about 1/. uz ur
zr = + , (41)
r z
and the heat diffusion vector qi is given by
3. Details of the numerical simulations
CP T Q Y
To assess accuracy of the analytical theory de- qz = + , (42)
Pr z Sc z
veloped in the previous section, we performed direct
CP T Q Y
numerical simulations of the hydrodynamic and com- qr = + . (43)
Pr r Sc r
bustion equations including chemical kinetics and
transport processes. In this section we are using di- Here = is the dynamic viscosity, CP is the heat
mensional variables. We investigated the case of an capacity per unit mass at constant pressure, and Pr and
axisymmetric flow described by the equations Sc are the Prandtl and Schmidt numbers, respectively.
The fuel mixture is assumed to be a perfect gas of
1
+ (rur ) + (uz ) = 0, (32) constant molecular weight m = 2.9 102 kg/mol,
t r r z with CP = 7Rp /2m and CV = 5Rp /2m, where Rp =
8.31 J/(mol K) is the perfect gas constant. The equa-
2
(uz ) + uz zz tion of state is
t z
1 P P= Rp T . (44)
+ r(uz ur zr ) = , (33) m
r r z
268 V. Bychkov et al. / Combustion and Flame 150 (2007) 263276
Similarly to our previous simulations [5,6,15,16], we than the tube radius, 20 < L/R < 100. We employed
used the initial pressure and temperature of the fuel a square grid with the grid walls parallel to the radial
mixture Pf = 105 Pa and Tf = 300 K. We have cho- and axial directions. The grid was uniform with the
sen the chemical parameters of the fuel mixture Ea , cell size 0.2Lf . It was demonstrated recently in [22]
Q, R , which provide strongly subsonic flame prop- that such a cell size is quite sufficient to simulate dy-
agation with the initial Mach number Ma Uf /cs = namics of a strongly curved flame front. Indeed, the
103 corresponding to the planar flame velocity Uf = characteristic length scale of the temperature profile
34.7 cm/s. In that case the flow is almost isobaric and inside the flame (the burning zone) is (45)Lf , while
thermal expansion is coupled to the energy release in the characteristic width of the active reaction zone is
the burning process as comparable to Lf [22]. Thus, taking a grid size of
0.2Lf , we obtain about 5 grid points inside the ac-
T Q
= b =1+ . (45) tive reaction zone and 2025 grid points inside the
Tf C P Tf
flame. For this reason, the grid used in the present
To imitate typical propane burning we chose the ex- simulations is sufficiently fine to resolve the inner
pansion factor = 8, the dynamic viscosity = flame structure even for a strongly elongated flame.
2.38 105 Ns/m2 , and the Prandtl number Pr = The simulation time step was much smaller than the
0.7. The flame thickness has been defined in a con- characteristic time of flame dynamics R/Uf .
ventional way as Similarly to the theory, we consider a tube with
ideally slip adiabatic walls and with one end closed.
Lf . (46) Boundary conditions at the side walls are
Pr f Uf
To avoid the Zeldovich (thermal-diffusion) instability T
ur = 0, uz = 0, =0
we assumed the coefficients of thermal diffusivity and r
fuel diffusion to be equal, i.e., the Lewis number equal at r = 0, R. (49)
to unity, Le Pr/Sc = 1 [3,23]. We chose the value
of the activation energy Ea = 7Rp Tb , which allows To avoid the influence of sound waves and weak
smoothing the reaction zone over a few computational shocks reflected from the open tube end, we applied
cells. Still, in the case of Lewis number Le = 1, nu- nonreflecting boundary conditions at the end. These
merical results do not depend on the magnitude of Ea conditions were tested in detail in [22]; they were
[3]. used also in our numerical works on flame acceler-
Similarly to [6,16], we used the axisymmetric hy- ation due to the Shelkin mechanism [5,6]. The initial
drodynamic Eulerian code developed in Volvo Aero. conditions were chosen in the form
The solver is robust and it was utilized quite suc-
cessfully in studies of laminar burning, hydrodynamic T /Tf = 1 + ( 1) exp ( R0 )/Lf ,
flame instabilities, and flame acceleration in tubes
if R0 , (50)
with nonslip at the walls according to the Shelkin
mechanism. The numerical scheme of the code and and T /Tf = , if < R0 , with
the computational method were described in detail in
[16]. We considered different tube radii in the domain T /Tf
Y= , (51)
5 < R/Lf < 30, which corresponds to relatively low 1
values of the Reynolds number related to the flame
propagation, where 2 = r 2 + z2 and R0 R is the initial radius
of a hemispherical flame front. The smaller R0 we
Uf R R use, the better we reproduce point ignition of a flame
Reflame = = = 1050. (47)
Pr Lf front; see Fig. 1. In the present simulations we chose
The Reynolds number related to the flow of the fuel R0 /Lf = 23. Equations (50) and (51) imitate the
mixture is much larger, hemispherical counterpart of the ZeldovichFrank
Kamenentsky solution [3]. The initial conditions at
2R uz
the open tube end are
Reflow = , (48)
and it may reach 103 104 at the end of the flame ac- = f , T = Tf ,
celeration, when the flame skirt touches the wall. For uz = 0, ur = 0, Y = 1. (52)
comparison, steady flows in tubes are usually laminar
at Reflow < 2 103 . Still, the values of Eq. (52) were not fixed during the
In order to reproduce an infinitely long tube, in the simulation run, and they may change because of the
present simulations we used a tube length much larger flame propagation.
V. Bychkov et al. / Combustion and Flame 150 (2007) 263276 269
(a) (b)
(c) (d)
(e) (f)
(g) (h)
Fig. 5. Flame shape for R = 20Lf at the time instants tUf /R = 0, 0.12, 0.21, 0.28, 0.32, 0.43, 0.64, 1.03. The colors designate
the temperature from the cold gas (blue) to the burnt matter (red). For interpretation of the references to color, in this figure
legend, the reader is referred to the web version of this article.
(a)
(a)
(b)
Fig. 6. Flame shape and the flow for R = 20Lf at the time
instants tUf /R = 0.12 (a), 0.28 (b).
Fig. 8. The scaled growth rate versus the tube radius. The Fig. 9. The growth rate versus the equivalence ratio for
markers show the results of numerical simulations. The solid propane flames for tube radii 2.5 and 5 cm. The filled mark-
line corresponds to the theory, Eq. (23); the dashed line ers show the experimental results [20]; the empty markers
present the model [20]. and the lines show the theoretical result, Eq. (23) calculated
using the data of Table 1.
Table 1
Parameters of the propaneair frame versus the equivalence ratio according to [28]
0.63 0.65 0.7 0.8 0.9 1.0 1.1 1.2 1.3 1.4 1.5 1.6
6.04 6.21 6.56 7.15 7.66 8.02 8.08 8.0 7.88 7.74 7.6 7.48
Uf (cm/s) 14.7 17.0 21.7 30.3 37.4 41.8 42.9 39.9 32.2 22.6 13.8 9.8
Fig. 12. Position of the flame tip by the end of the acceler- Fig. 13. Position of the flame tip versus time according
ation versus the tube radius. The markers show the results to the theory (dashed line), Eq. (21), experiments [20]
of numerical simulations; the solid line corresponds to the for the propaneair mixture with = 0.7, and modeling.
theory, Eq. (22). The marker indicates the time instant when the flame skirt
touches the wall.
and we cannot compare the respective numerical and
theoretical results to the experimental ones. Fig. 12
shows the height of the flame tip till the end of the
flame acceleration obtained in the numerical simula-
tions and predicted by the theory for = 8, Eq. (22).
This plot looks qualitatively similar to the previous
one: the numerical results for the tip height increase
with the tube radius (with decreasing influence of
flame thickness) and approach the theoretical predic-
tions. Fig. 13 presents the tip position for a propane
air flame of equivalence ratio = 0.7 obtained ex-
perimentally [20]. The dashed line shows theoretical
predictions of Section 2, Eq. (21), for = 6.56 cor- Fig. 14. Characteristic time instants of the flame evolution,
responding to = 0.7. We can see that the theory tsph , twall , and ttulip , versus the ratio R/Uf (s). The markers
is in excellent agreement with the experiments. The show the experimental results [20]; the lines correspond to
marker indicates the time instant when the flame skirt the theoretical formulas, Eq. (17), (18), and (59), with = 1.
touches the wall, with the tip position Zwall = R, takes the average value 7.28.
Eq. (22). Strictly speaking, the theory of Section 2
holds only up to this time instant. Still, as we can theoretical evaluations of these two time instants are
see from Fig. 13, the theory describes the tip posi- given by Eqs. (17) and (18). As for the numerical re-
tion quite well even beyond that limit until a tulip sults, it is difficult to extract tsph from the numerical
flame is formed with temporal retreat of the axial simulations because of the vague definition of that in-
point at the flame front. For comparison we show also stant. In the experiments [20] this time has not been
the results of numerical simulations in Fig. 13. The measured either; instead, it was calculated on the ba-
numerical simulations provide qualitatively the same sis of the model Eqs. (1)(3) using the formula
picture. However, one should not expect quantitative
R
agreement in that case because of the inevitable nar- tsph = twall ln(Zwall /R). (53)
row tubes in the simulations. Besides, the simulations 2Uf
assumed = 8, which is different from the experi- In contrast, the instant twall is defined quite well, and
mental data of Fig. 13. it may be compared to the theory and the experiments.
Another interesting question concerns time limits Fig. 14 compares the theoretical predictions and the
of the acceleration: it starts when the spherical flame numerical results to the experimental data of [20].
develops into a finger-shaped front at tsph , and it At that point we have to say that different equiva-
stops when the flame touches the wall at twall . The lence ratios of the propaneair flame correspond to
V. Bychkov et al. / Combustion and Flame 150 (2007) 263276 273
Fig. 15. Position of the flame skirt versus time according to Fig. 16. Correlation of the skirt velocity with the value
Eq. (54), experiments [20] for the propaneair mixture with Zwall /R. The markers show the experimental results [20];
= 0.7 (markers), and modeling. the line corresponds to Eq. (54) with = 1.25.
the different expansion factors = 68 and, there- The characteristic experimental evaluations for these
fore, lead to somewhat different values for tsph , twall . values were twall 0.26R/Uf , ttulip 0.33R/Uf ,
To plot the theoretical lines we took an intermediate tinv 0.07R/Uf . We point out that the last value
value = 7.23 calculated as an average for all exper- correlates rather well with the inverse growth rate
imental points. Still, even with this inevitable reason 1 R/Uf . The reason for such a correlation may
for scattering of the experimental points, the theory be demonstrated within the following semiqualitative
agrees well with the experiments. model. As the skirt position moves along the wall, the
As soon as the flame touches the side wall of the burnt gas velocity, Eq. (7), modifies roughly as
tube, the skirt of the flame front sweeps along the wall
at high speed because of the small angle between the v2 = A2 ( skirt )
2( 1)( skirt )
flame front and the wall. Fig. 15 shows the skirt posi-
( skirt ), (55)
tion versus time obtained experimentally for = 0.7
in [20] and in the numerical simulations. Similarly to and Eq. (20) reduces to
Fig. 13 for the flame tip, the numerical results under- dtip
estimate the skirt velocity, presumably because of the
tip 2 ( wall ) + , (56)
d
influence of the finite flame thickness. It was pointed
out in [20] that during the interval of flame decelera- taking into account Eq. (54). Because of the initial
tion the skirt velocity is almost constant, and it corre- conditions tip (wall ) = , Eq. (22), we can neglect
lates rather well with the value Uf Zwall /R. The last the last term in Eq. (56) in the limit of 1 1.
value may be calculated on the basis of our theory in Then, integrating (56), we find that
Section 2 as 2 ( 1)Uf , which gives the skirt
velocity tip = ( 1) exp ( wall )
+ ( wall ) . (57)
Uskirt = 2 ( 1)Uf , (54)
The instant ttulip corresponds to Ztip = Zskirt or
with the factor comparable to unity. The physical dtip /d = 0, and the interval of inversion tinv =
meaning of is that it compares the skirt velocity ttulip twall is calculated from (57) as
during the deceleration to the characteristic parameter
of velocity dimension Uf Zwall /R during the flame
acceleration. In Fig. 15 we took = 1.25 to obtain Uf tinv /R = inv = 1 ln . (58)
1
the best agreement of Eq. (54) with the experiments;
Uskirt is calculated from the slope of Zskirt . However, The evaluation (58) for tinv is simpler than the respec-
in general may depend on the expansion factor . tive formulas in [20], and it demonstrates clearly the
Fig. 16 compares the skirt velocity measured experi- correlation tinv 1 R/Uf . Still, one has to remem-
mentally to the theoretical value for Uf Zwall /R; the ber that calculations (55)(58) are only a qualitative
solid line presents Eq. (54) for = 1.25. Indeed, we model based on the empirical formula (54). There-
can see a very good correlation between the experi- fore, in reality, one should interpret (58) as another
mental data and Eq. (54). Eventually the skirt catches correlation of the form
up with the tip, and the flame front becomes first pla-
tinv = 1 R/Uf (59)
nar and then inverted (or tulip-shaped). The time in-
stant of inversion was called ttulip in [20], and the time with the coefficient comparable to unity. The eval-
interval needed for the inversion is tinv = ttulip twall . uation (59) is compared to the experimental data in
274 V. Bychkov et al. / Combustion and Flame 150 (2007) 263276
shape with the surface area Sw / R 2 = 2.4 exceed- the most interesting stages of flame dynamics: hemi-
ing noticeably the respective surface area of the sta- spherical expansion, acceleration of the finger-shaped
tionary concave flames Sw / R 2 = 1.11.2; see [16]. flame, rapid deceleration when the flame skirt sweeps
The maximal flame curvature in the tulip flame cor- along the tube side wall, and inversion of the flame
responds to the local (in time) maximum of the flame shape, which may be also interpreted as a tulip
surface area in Fig. 7a achieved at Uf t/R 0.6. Later, flame.
the strongly concave flame collapses again to the pla- In the present paper we considered only the case of
nar flame shape, which may eventually develop to a adiabatic tube walls. Losses to the walls may reduce
stationary DL curved flame like that obtained in [16]. the effective thermal expansion and make the flame
To conclude the discussion, we believe that the notion acceleration noticeably weaker. This is a subject for
of tulip flame is misleading, since it embraces too future work.
many combustion phenomena of different origin. In-
stead, it would be much better to talk about curved
flames, indicating the reason for the curved shape. Acknowledgments
A particular example is inversion of the curved flame
shape because of a shock as in [32,33] or because of The authors thank Geoffrey Searby for the experi-
flame deceleration as in [20] and in the present pa- mental data of Figs. 9 and 1316 and Mikhail Ivanov
per. for useful discussions. This work has been supported
in part by the Swedish Research Council (VR) and by
the Kempe Foundation.
5. Summary
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[22] V. Akkerman, V. Bychkov, A. Petchenko, L.E. Eriks- 297.
son, Combust. Flame 145 (2006) 675. [30] E.E. Meshkov, Fluid. Dynam. (USSR) 4 (1969) 101.
[23] G.I. Barenblatt, Ya.B. Zeldovich, A.G. Istratov, Prikl. [31] G. Markstein, in: G. Markstein (Ed.), Non-Steady
Mech. Techn. Fiz. 2 (1962) 21. Flame Propagation, Pergamon, London, 1964, p. 15.
[24] H. Genoche, in: G. Markstein (Ed.), Non-Steady Flame [32] V. Bychkov, Phys. Fluids 10 (1998) 2669.
Propagation, Pergamon, London, 1964, p. 107. [33] O. Travnikov, V. Bychkov, M. Liberman, Combust.
[25] M. Gonzalez, R. Borghi, A. Saouab, Combust. Flame Sci. Technol. 142 (1999) 1.
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