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VOLUME 50 T I'EBRUARY 198) NUMBER 6

Propagating Pattern Selection


G. Dee and J. S. Langer
Institute for Theoretical Physics, University of California at Santa Barbara, Santa Barbara, California 93106
(Received 6 December 1982)
Pattern selection is discussed in regard to a situation where a stable, nonuniform state of
a nonlinear dissipative system propagates into an initially unstable, homogeneous region.
The velocity of the propagating front and the wavelength of the pattern formed behind the
front are determined by a marginal-stability criterion. The special system studied here
has a I,yapunov functional, but the periodic state which propagates is not the one which min-
imizes the functional.
PACS numbers: 05.70. Ln

Development of a meaningful theory of natural derivation has been discovered.


pattern selection requires models of pattern- The first group of pattern-forming phenomena
forming mechanisms that are simple enough to mentioned above has the common feature that
be understood in detail. Real systems are in- periodic structures are emerging in translational-
trinsically complex and exhibit a variety of re- ly symmetric systems. A particular mechanism
sponses to differing experimental situations. One for pattern formation in such systems, which we
would like, for example, to predict the periodici- shall call "pattern propagation, " has some simi-
ties of Rayleigh-Benard convection patterns, ' of larity to the dendritic process. ' Consider an
cellular solidification fronts, ' cellular flame initially structureless system which is "quenched"
fronts, ' etc. The basic difficulty is that the so that it becomes uniformly unstable against
steady-state descriptions of each of these systems pattern-f orming deformations. A perturbation
admit whole bands of linearly stable states; yet, which at first is confined to a small region will
at least under some conditions, unique states are grow locally into a well developed pattern~on-
selected in real experiments. It will ultimately vective rolls, cellular structures, etc. and this
be important to understand whether, or under pattern will spread out into the rest of the space.
what circumstances, pattern formation in such This pattern may spread by propagating at a well-
, systems is an intrinsic property of the systems defined velocity, the front of the pattern looking
themselves or, perhaps, depends sensitively on much like the tip of a dendrite which generates
initial configurations, boundaries, or externally an array of side branches behind it as it moves.
imposed perturbations. ' A picture of such a pattern front is shown in Fig.
A particularly striking example of the pattern- 1. The crucial questions are the following: What
tic solidification. "
selection problem occurs in the theory of dendri-
In this case, it appears that
the naturally selected states are those which sit
is the speed of the front? What is the wavelength
of the pattern which is stabilized behind this
front?
just at the margin of instability. Although quali- An instructive example is a nonlinear diffusion
tative arguments have been advanced in favor of
this principle of marginal stability, no systematic literature of mathematical biology. ' "
equation which has been much discussed in the
We shall

1983 The American Physical Society 383


VoLUM+ 50~ +UMg~R PHYSICAL REVIEW LETTERS 7 FEBRUARY 1983

who prove that all initial states v(x, t = 0) which


lie within the strip 0 v - -1 ich o not vanish
which
, w
everywhere, and which decrease at least f t
in e +x direction will form propagating
i,
fronts with c =2. That is thee b asin of attraction
or the state v , is overwhelmingly bigger than
that for any other and , in particular, contains all
the physically achievable initial per turbations
OQ which are of bounded exte n t . Th is, then, is an
example of a sharp selection mechanism
This selected state is marginally stable. The
i i+~ " is used here in just the same
term "stabili
I I

pp p Boo X in e rame of
FIG. 1. Fro r d eter-
Front portion of a propagating paatt em reference ce movi
moving with the front and ask whether
mined e ==0.9. The oscillatory part of
q. ( 4 for
byy Eq. an initial 1y lococalized perturbation, observed at
the pattern on the left is stationar in the l b a fixed point in that framee, wi'll grow or decay.
rame, and new oscillations arise as the envelope of perturbation which decays ays is considered stable
the pattern moves to the right. Inset: the local wave
even if it generates a growing disturbance like
number k as a function of x fo r th e entire system.
e,
a sidebraneh which moves away from its point
of origin near the tip. The d e t ai'l e d analysis of
consider at first only a specially symmetric ver- st
thee stability spectrum for Eq. (1) will be pub-
sion, viz. ished elsewhere. For preesen t purposes, we
sU/si = 8'v/sx'+u u' (1) shall use an intuitively appealining but u over simpli-
ie pic ure which we shall prese sen t in such a wa
which is also well known in the pph ysics 1't
i erature
that it can be applied too a wi d er class of models
as a model for phase transformations. Stable
than that described in Eq. (1).
states of this system occur aat v=+,
v =+ 1 and an un-
' Consider a localized pert ur b a t ion imposed on
a e state at v=0. The situation f terest
sstabl an otherwise uniform unstable s stem
is one in which the unstable state v =0 is trans- small dis isturbances,
u we can linearize e ua-
ize thee equa-
formed into sa y, = I at a front moving at speed tion of motion ion, make
m a Fourier transfo rma t'ion,
c. This steady-state front must be described b '
obtain a dispersion relationn for or thee amplifiea-
=x ct, which is a solutioion
of
tion ratee ~ e as a function of wave number k. After
a long time t, and at a larg e d is t ance x away
0 = &v, /sx" +c &~, /W'+ v C o C ' fro
rom the initial disturbance th e perturbation
will have the form exp[it*x+ x + ~ (k*'tf, where 4*
with the boundary conditions v,C -1 at x'- ~ is e point of stationary phase in thee complex k
vc -0 x'-+
at
ane. If we observe this perturbation at a mov-
p lane.
Solutions of ~2& exist for all positive values of c.
ing position x =ct, then we should ou a
bee able to
To see this, note that (2) can be interpreted as
choose c lar arge enough that we outrunn th e pertur-
the mechanical equation of m ot'ion f or a particle
bation, that a is, we should
h see a decaying expo-
of unit mass whose "displacement"
ime ' x'. The particle is undergoing
nential in time. e. 'n this sense, c is a stabilizing
parameter. The marginal- t b'l'
damped motion with damping constant a o-
an c in apo-
is simply the conjecture that the natural veloci
.

o,
,v, he relevant trajectories are
,c, is at for which this

c,t,
those in which the particle starts 'th zero speed
exponential neither grows nor no d ecays. Ther ef ore
from the potential maximum um a vc= 1= I and falls to c should be obtained by solving
the minimum at v C = 0. For & 2 th e motion is
overdamped, and the front v, ~~x j is monotone de-
ic*+dcu/du*=0; Re1ic*a'+su(e*)] =0
creasing. For the underdamped ease, c & 2, the
ci a es as it approach-
forward part of the front oscillate
es v, ==0 Note that this analysis works cor ree tl y t o give c*
A defin'
initive mathematical discussion of Eq. (1) when &u = 1 k' as in the case of Eq. (1).
has been published by Aronson and Neinber er ' A much more interesting case to consider is
VOLUME 50& NUMBER 6 PHYSICAL REVIEW LETTERS 7 FEBRUARY 1983

the equation
&u/&t = [ e ( s'/Bx'+ 1)'] u u', (4)
Here, & is a control parameter introduced in
such a way that the state u =0 becomes unstable
when ~ becomes positive. The restabilized sta-
tionary solutions of (4), for any fixed e in the
range 0 ca ~1, are periodic functions with funda-
mental wave numbers k occurring in bands of
finite width in the neighborhood of k -1. For
small e, (4) can be approximated by an amplitude
05
l.
equation by writing
u(x t ) =- (-' e)"W(X T)e i" + (-' W+(X T)e - '"
e)" l I

0-I 0.2 DX

where X = 2E x and ~= EI,. Then the amplitude to 6


W satisfies
FIG. 2. Scaled velocity c*/4+e as a function of the
BW/BT= & W/BX +W i Wi W+O(e ). (6) control parameter e. Inset: the extrapolation to van-
This is the same as (1) except that W may be ishing grid spacing used in estimating q* for e =0.9.
complex. There are strong reasons for believing
that localized initial conditions must evolve ac-
pattern, this flux must be conserved and must be
cording to (6) into propagating states in which
equal to k, c* in the bulk. Thus, we predict
the phase of 8' becomes very nearly constant,
so that the theorems of Aronson and Weinberger k, = Q/c*. (6)
are applicable. This leads to the prediction tha, t, For example, for a=0. 9 we find c*/e' '=4. 546,
to lowest order in c, c*= 4&' '. The correspon- Rek*=1.1758, A=4. 643, and k, =1.076.
dence between (4) and (1) via the amplitude Eq. These predictions for c* and ky have been
(6) does not prove, but makes it plausible, that checked by direct numerical solution of Eq. (4).
pattern propagation in this more complicated Our procedure is straightforward; we start with
model occurs at a sharply defined speed. a localized perturbation and watch it evolve as
The simplified marginal-stability theory sum- shown in Fig. I. Our results for the propagation
marized in (3) may be used to compute the func- speed are 'generally consistent with the predicted
tion c*(e) throughout the physically interesting c (e) shown in Fig. 2. The inset in that figure
range (0&a&1) by setting &u(k) =e-(k'-I)'. The shows measured values of c for ~ = 0.9 at three
results are shown in Fig. 2. This theory may different grid sizes, with our proposed extrapola-
also be used to predict the wavelength of the pat- tion indicated by the dashed lines. The error
tern which emerges behind the front. In doing bars indicate only the scatter in our data and not
this, it is helpful to look at the wave form in Fig. any estimate of systematic error, except that
I, which is a computer-generated solution of Eq. the bar for the point at the smallest grid size is
(4) for e = 0.9. The fully developed pattern has skewed because the speed of the front seemed
a, wa. ve number k, and is stationary in the fixed
still to be increasing slowly at the end of this
frame of reference. Alternatively, the pattern run.
may be visualized as moving with velocity -c*
The inset in Fig. I shows the local wave number
in the frame of reference in which its envelope
k as a function of x for the entire system whose
is at rest. Ahead of the front, the pattern is pre- front is shown in the main part of that figure.
dicted by (3) to have a wave number Rek* and to
Note that the wave number in the body of the pat-
be oscillating at a fixed point in the moving frame, tern has settled down accurately to.the predicted
with an angular frequency
kg Ahead of the f ront, k passes thr ough Re@*
0 =Im[ik*c *+u(k *) ]. (7) and the amplitude of the wave form decreases
This frequency may be interpreted as a flux of rapidly. The variation of k near x =0 is a vestige
nodes moving in the -x direction relative to the of the initial transient which has been trapped
envelope. As long as nodes are not created or behind the front and is slowly disappearing diffu-
destroyed when they pass through the front of the sively. One of the reasons that we must use long
VOLUME 50, +UMBER 6 PHYSICAL REVIEW LETTERS 7 FEBRUARY 1983

computer runs to evaluate c is that we must allow of (4). The Eckhaus instability, where the phase-
enough time for the front to become well sepa- diffusion constant for the bulk pattern vanishes,
rated from this transient. occurs at k = 1.25 for e = 0.9. Thus, the selected
The results of this investigation are encourag- wave number in this case definitely does not oc-
ing in the sense that we seem to have found a cur near a marginal instability of the bulk pat-
sharp selection mechanism which is an intrinsic tern, as has been suggested in another context. "
property of the system, independent of detailed This work was supported by the U. S. Depart-
initial conditions, boundary effects, or external ment of Energy, under Contract No. DE-AM03-
perturbations. On the other hand, these results 765F00034 and by the National Science Founda-
are discouraging to hopes of finding universal tion under Grant No. PHY77-27084. The research
selection criteria. In the first place, the mecha- was carried out as part of an Institute for Theore-
nism described here depends only on linear prop- tical Physics program on nonequilibrium phe-
erties of the unstable part of the system, and we nomena, and many of the early ideas were devel-
know that this cannot be true in general. For oped in collaboration with E. Ben-Jacob,
example, the addition of a term of the form v' H. Brand, and L. Kramer. The authors are
to the right-hand side of (1) invalidates the simpli- also indebted to R. Ball, J.
-P. Eckmann, P. C.
fied version of the marginal-stability hypothesis Hohenberg, and G. Schon for important contribu-
summarized in (3). It turns out that marginal tions.
stability is still correct, but the instability which
controls the speed of propagation is a localized
deformation of the front which appears only in 'A. Schluter, D. Lortz, and F. Busse, J. Fluid Mech.
the fully nonlinear analysis. We do not know 23, 129 (1965); A. C. Newell and J. C. Whitehead, J.
under what circumstances such a nonlinear effect Fluid Mech. 38, 279 (1969).
might occur in a pattern-forming model like (4), 'J. S. Langer, Rev. Mod. Phys. 52, 1 (1980).
but we see no reason to exclude this possibility. G. I. Sivashinsky, 'Instabilities, Pattern Formation,
An even more serious point to recognize is that
"
and Turbulence in Flames, to be published.
4L. Kramer, E. Ben-Jacob, H. Brand, and M. C.
there exists a Lyapunov function E(uj for Eq. (4),
Cross, Phys. Rev. Lett. 49, 1891 (1982).
and that the selected wave number k, is not the 5J. S. Langer and H. Miiller-Krumbhaar, Acta Metall.
one which minimizes I'. That is, given reason- 26, 1681, 1689, 1697 (1978).
able boundary conditions of the kind used here, 6J. S. Langer and H. Muller-Krumbhaar, Phys. Rev.
we can write (4) in the form A 27, 499 (1982). Pattern propagation has also been
observed in numerical simulations by Kramer et al. ,
Bu/Bt = 5E/5u, Ref. 4, who have studied both the dendritic model and
coupled reaction-diffusion systems.
dX ~ +2 1 CQ +gQ ~R. A. Fisher, Ann. Eugenics 7, 355 (1937).
BA. Kolmogoroff, I. Petrovsky, and N. Pisconnoff,

(9) Bull. Univ. Moscow, Ser. Internat. , Sec. A 1, 1 (1937).


~D. Q. Aronson and H. F. Weinberger, in Partial Dif-
and note that dE/dt-0. For a=0. 9, E has its ferential Equations, Lecture Notes in Mathematics Vol.
absolute minimum at the stationary state with 446, edited by J. A. Goldstein (Springer, New York,
fundamental wave number k =0.998, which differs 1975), p. 5.
from k, =1.076 by an amount which is well beyond 'OD. Q. Aronson and H. F. Weinberger, Adv. Math.
our numerical uncertainty. Thus, patterns which 30, 33 (1978).
form by propagation will not be the same as those
"J. Swift and P. C. Hohenberg, Phys. Rev. A 15, 319
(1977).
which are most stable in the presence of, say, ' Y. Pomeau and P. Manneville, J.
Phys. Lett. 40,
thermal fluctuations. 609 (1979). See also M. C. Cross, P. Q. Daniels, P. C.
Finally, we remark that both k, and Rek* lie Hohenberg, and E. D. Siggia, to be published.
well within the band of stable stationary solutions '3J. S. Langer, Phys. Rev. Lett. 44, 1023 (1980).

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