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Abstract
Electrical characteristics of a 1 cm-long free-burning atmospheric-pressure argon arc are
calculated by means of a model taking into account the existence of a near-cathode
space-charge sheath and the discrepancy between the electron and heavy-particle temperatures
in the arc column. The computed arc voltage exhibits a variation with the arc current I similar
to the one revealed by the experiment and exceeds experimental values by no more than
approximately 2 V in the current range 20175 A. The sheath contributes about two-thirds or
more of the arc voltage. The LTE model predicts a different variation of the arc voltage with I
and underestimates the experimental values appreciably for low currents but by no more than
approximately 2 V for I 120 A. However, the latter can hardly be considered as a proof of
unimportance of the space-charge sheath at high currents: the LTE model overestimates both
the resistance of the bulk of the arc column and the resistance of the part of the column that is
adjacent to the cathode, and this overestimation to a certain extent compensates for the neglect
of the voltage drop in the sheath. Furthermore, if the latter resistance were evaluated in the
framework of the LTE model in an accurate way, then the overestimation would be still much
stronger and the obtained voltage would significantly exceed those observed in the experiment.
(Some figures may appear in colour only in the online journal)
0022-3727/12/355201+10$33.00 1 2012 IOP Publishing Ltd Printed in the UK & the USA
J. Phys. D: Appl. Phys. 45 (2012) 355201 M S Benilov et al
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J. Phys. D: Appl. Phys. 45 (2012) 355201 M S Benilov et al
It was found in [25] that the electric power deposited into involves the equation of heat conduction in the cathode body
the near-cathode sheath is transported not only to the cathode coupled through a boundary condition with a system of
but also to the quasi-neutral plasma (arc column), an effect transcendental equations describing current transfer through
that cannot be described by LTE models. This effect has been the near-cathode layer. The motion of ions in the space-
independently confirmed in [24]. Obviously, this transport can charge sheath is assumed to be collisionless and is described
substantially reduce the resistance of the part of the arc column kinetically. (This description is expected to be reasonably
adjacent to the sheath. In order to describe this transport, one accurate also in the case of moderately collisional sheaths,
needs to take into account not only the presence of the sheath, although not in the case where the ion motion in the sheath is
but also eventual discrepancy between the electron and heavy- strongly collisional, which occurs, for example, in very-high
particle temperatures Te and Th in the arc column, at least in the pressure high-intensity discharge lamps operating under the
part adjacent to the near-cathode sheath. Both effects, which pressure of the order of 100 bar or higher.) The ionization
are discarded in LTE models, have been taken into account layer is described by means of fluid equations. Calculation
in [24, 25]. of distribution of potential in the cathode has shown that the
Thus, one may hypothesize that LTE models substantially variation of potential in the cathode does not exceed 0.4 V
overestimate the resistance of the part of the arc column that is for conditions considered in this work, therefore the voltage
adjacent to the near-cathode sheath and this overestimation to drop and Joule heating in the cathode body are neglected. The
a certain extent compensates discarding the voltage in the near- voltage drop Ucl across the near-cathode layer is assumed to
cathode sheath. This question clearly deserves an elaboration. be the same at different points of the arc attachment.
Another question that needs to be analysed is the effect of The arc column is computed by means of a two-
deviations from LTE on the resistance of the bulk of the arc temperature (2T) hydrodynamic model, which accounts for
column. inequality of the electron and heavy-particle temperatures,
In this work, a model similar to that in [25] is employed for Te = Th , but assumes the ionization equilibrium and quasi-
finding electrical characteristics of a high-current atmospheric- neutrality. The model comprises the NavierStokes equations,
pressure argon arc. Also performed are simulations by equations of energy for the heavy particles and the electrons,
means of an LTE model. The arc voltage predicted by equation of continuity of electric current supplemented with
both models is compared with the experimental data [26]. Ohms law and Amperes law for the self-induced magnetic
Also considered is the question of error introduced into the field. The anode is simulated by means of a model comprising
evaluation of the resistance of a near-cathode plasma by equations of heat conduction and continuity of electric current
algorithms conventionally used in LTE models. supplemented with Ohms law. Note that variations of
potential in the anode are in fact very small (of the order of
2. The model 1 mV); however, the current continuity equation is nonetheless
maintained in the model for technical reasons.
The model used in this work is similar to the one of [25] The coupling between the sub-domains is as follows. Let
and may be briefly described as follows. The whole system us use Th for the heavy-particle temperature, where the arc
comprising the arc and the electrodes is divided into three sub- column and the near-cathode plasma layer are concerned,
domains simulated by means of separate models: the cathode and for the temperature of the electrode material, where the
and the near-cathode plasma layer, the arc column, the anode; electrodes are concerned. At the interface between the arc
the near-anode plasma layer is discarded. The cathode and column and the near-cathode layer, the temperature Th is
the near-cathode plasma layer are described by means of the assumed to be continuous, as well as the electron temperature
model of nonlinear surface heating. A summary of equations Te , the electrostatic potential , and the normal component
of the model can be found in [27]. A more detailed description jn of the electric current density (here and further n is a
and an online tool for simulation of the diffuse and spot modes coordinate measured from the electrode surface normally to
of current transfer and their stability based on this model can it in the direction into the plasma). Note that variations of
be found in [23]. Detailed presentations of different aspects of heavy-particle temperature across the near-cathode layer are
the model, as well as its detailed experimental validation, can neglected; we recall that the near-cathode plasma layer, which
be found in [13] and original works cited therein. is of interest for this work, comprises the sheath and the
In brief, the model of nonlinear surface heating may be ionization layer and its thickness is of the order of 1 m or
introduced as follows. The model exploits the following smaller. Therefore, the continuity of Th means that the heavy-
feature of the physical picture accounting for the existence particle temperature on the arc column side of the interface
of the sheath: the electrical energy deposited by the arc equals the temperature of the cathode surface.
power supply in a sheath with a voltage of 1015 V is quite At the interface between the arc column and the anode,
significant, and it is a part of this energy that is transported Th , and jn are assumed to be continuous. The density of
to the cathode and heats it; as a consequence, the plasma flux of energy from the arc column to the anode is evaluated
cathode interaction is governed by processes occurring in a as the sum of heat fluxes transported by the heavy particles
thin near-cathode plasma layer comprising the sheath and the and the electrons and of the additional term jn (Af + 2.5kTe )/e
adjacent ionization layer, and to the first approximation the (here Af is the work function of the electrode material), which
plasmacathode interaction is unaffected by the arc column. accounts for heating of the anode surface due to condensation
In mathematical terms, the model of nonlinear surface heating of electrons.
3
J. Phys. D: Appl. Phys. 45 (2012) 355201 M S Benilov et al
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J. Phys. D: Appl. Phys. 45 (2012) 355201 M S Benilov et al
-10 160
I = 40 A
2T-sheath
model
2
10
(a) 12 14 16 18 z (mm)
20 22 (b) 12 14 16 18 z (mm)
20 22
8
10 (103 S m-1) 10 -jz (A m-2)
160
8
Figure 3. Distributions of electrical parameters on the axis of the arc column; I = 40, 160 A. (a) Electrostatic potential; (b) axial electric
field and (c) electrical conductivity of the plasma. The data referring to the 2T-sheath model for I = 160 A are represented by a dotted line
in order to distinguish in the black-and-white print from the line representing the data for I = 40 A. (d) Axial current density.
field; however, this region is narrow and unimportant for the latter is seen also from figure 3(d). The temperature in the arc
following.) core is also lower. Thus, the arc core as described by the 2T-
As far as the bulk of the arc column is concerned, the sheath model is colder and wider, hence the energy losses from
reason for values of |Ez | predicted by the LTE model being it are lower. The latter means that the arc column consumes a
higher is as follows. In figure 6, radial distributions of lower electrical power, i.e. for the same arc current the axial
parameters of the arc column in the midplane of the arc, z = electric field is lower.
17 mm (i.e. halfway between the electrodes), are shown. In the There is an additional reason for values of |Ez | predicted
framework of the 2T-sheath model, the electron temperature by the LTE model being higher which comes into play in the
and, consequently, electrical conductivity of the plasma in immediate vicinity of the cathode or, in the framework of the
the arc fringes are higher than those for the same I in the 2T-sheath model, of the interface separating the column from
framework of the LTE model. The current density is higher in the near-cathode layer. This reason is seen from figure 3(c):
the arc fringes and correspondingly lower in the arc core; the calculated by means of the LTE model rapidly decreases
5
J. Phys. D: Appl. Phys. 45 (2012) 355201 M S Benilov et al
-3 jn (107 Am-2) (V) 0 see that the arc column contributes about one-third or less of the
arc voltage and the rest is contributed by the near-cathode layer,
(2T)
i.e. essentially by the space-charge sheath. Uarc (I ) decreases
160 for lower currents, passes through a minimum at I = 100 A,
and slowly increases for higher currents.
-2 I = 40 A Also shown in figure 5 are experimental data on the
(exp)
arc voltage, Uarc , taken from [26]. (The authors [26]
distinguish two forms of arc attachment to the cathode:
160 -5
diffuse and contracted. However, the difference between
the corresponding arc voltages is below 1 V. We note for
-1 definiteness that the values shown in figure 5 refer to the
40 (exp) (2T)
diffuse form.) The dependence Uarc (I ) is similar to Uarc (I ),
although the minimum occurs at a higher current I = 140 A.
jn The numerical values are also not very different: Uarc (2T)
exceeds
(exp)
Uarc by less than 1 V at lower currents and by about 2 V at
0 -10 higher currents.
0 1 2 3 s (mm)
4 5 In the framework of the LTE model, the total arc voltage
(LTE)
coincides with the arc column voltage Uac . The dependence
Figure 4. Distributions of potential and normal current density (LTE) (2T) (exp)
along the interface separating the arc column and the near-cathode Uac (I ) is of a different character than Uarc (I ) and Uarc :
(LTE) (LTE)
layer; I = 40, 160 A. Uac (I ) monotonically increases for all currents. Uac is
(2T) (exp)
lower than both Uarc and Uarc ; the difference is significant
20 Voltages (V) for lower currents but decreases with current and is reduced to
no more than approximately 2 V for I 120 A.
U (2T)
arc
16 4. Effect of numerics over the arc voltage predicted
by the LTE model
U (exp)
arc
12 Sensitivity with respect to details of numerical grids in the
vicinity of the cathode is a known issue for LTE models of
high-pressure arc discharges. In this connection, computations
Ucl
have been performed in which the code describing the arc
8 U (LTE)
ac column and the anode (and, in the case of the LTE model, also
U (2T)
ac the cathode) was operated on a series of grids successively
refined in the vicinity of the cathode. The number of control
4 volumes on the axis of the arc column in each of the grids
0 40 80 120 I160
(A) 200 and positions (z-coordinates) of the two main grid points, i.e.
centres of control volumes closest to the cathode are indicated
Figure 5. Uac(2T) , Uac(LTE) : arc column voltage evaluated by means of, in table 2. Note that the simulations described in section 3
respectively, the 2T-sheath and LTE models. Ucl , have been performed on grid 1 for the 2T-sheath model and on
(2T)
Uarc = Uac(2T) + Ucl : voltage drop in the near-cathode layer and arc
(exp) grid 4 for the LTE model.
voltage evaluated by means of the 2T-sheath model. Uarc :
measured arc voltage [26].
An example of the results is shown in figure 8. One can
see from figure 8(a) that the use of different grids does not
in this vicinity, while calculated by means of the 2T- appreciably affect the results given by the 2T-sheath model.
sheath model rapidly increases. This is a consequence of In contrast, results given by the LTE model indeed depend
different behaviour of the temperatures, which is shown in on the grid, especially in the vicinity of the cathode. This effect
figure 7. Both the heavy-particle temperature Th and the is clearly seen in figure 8(b), which represents a magnification
LTE plasma temperature T decrease in the direction to the of the relevant part of figure 8(a), and is non-negligible. There
cathode (note that at z = 12 mm both Th and T equal the is no way to eliminate this dependence by means of a further
temperature of the cathode surface, which does not exceed refinement of the grid in the vicinity of the cathode, since such
4000 K). However, the electron temperature Te , which governs refinement leads to the loss of convergence. The reason for
the plasma conductivity in the 2T-sheath model, increases, the problem is well known: it is a steep decrease of the LTE
which is due to the transport into the arc column of electric plasma temperature in the vicinity of the cathode, which causes
power deposited into the near-cathode sheath [24, 25]. a dramatic variation of the plasma conductivity. The latter is
The total arc voltage in the framework of the 2T-sheath illustrated by table 3. Here, indices w, 1 and 2 are attributed
(2T)
model, Uarc , is obtained by adding the arc column voltage to values of the corresponding quantities at, respectively, the
(2T)
Uac and the voltage drop in the near-cathode layer, Ucl . These centre of the front surface of the cathode (point C in figure 2)
voltages as functions of current are shown in figure 5. One can and the first and second main points of each grid on the axis
6
J. Phys. D: Appl. Phys. 45 (2012) 355201 M S Benilov et al
16 Te,Th,T (103 K) 8
T (103 I = 160 A
160 S m-1)
12 6
160
8 Te 4 40
LTE model
I = 40 A Te
Th
40 2T-sheath
4 2 model
T Th
0 0
0 2 4 6 r (mm)
8 10 (b) 0 2 4 6 r (mm)
8 10
(a)
-6 jz (106 Am-2)
I = 160 A
-4
LTE model
160
-2
2T-sheath
40 model
40
0
(c) 0 2 4 6 r (mm)
8 10
Figure 6. Radial distributions of parameters of the arc column in the midplane of the arc. I = 40, 160 A. (a) Te , Th : electron and
heavy-particle temperatures (2T-sheath model), T : the plasma temperature (LTE model). (b) Electrical conductivity of the plasma. (c) Axial
current density.
20 Te,Th,T (103 K)
of the arc (positions of these points are given in table 2); Tw
and w are determined by means of linear extrapolation of
T
Te distributions of the temperature and potential at the axis of the
(LTE)
cathode (note that the values of Uac shown in figure 5 and
15 160 the values of potential at z = 12 mm shown in figure 8(b) are
also determined in this way); w is evaluated in terms of Tw by
Te T means of the data [31]. There is a two- to five-fold variation of
10 between the second and first main grid points and a variation
Th of five orders of magnitude between the first main grid point
I = 40 A
and the cathode surface.
Th
In the SIMPLE numerical algorithm being used, transport
5
coefficients are assumed to be constant in each control
volume; an assumption clearly unsuitable as far the electrical
conductivity of the plasma near the cathode is concerned. Note
0 that transport coefficients on the interface between adjacent
12 12.5 13 z13.5
(mm) 14 control volumes are evaluated as a harmonic mean value (e.g.
[30, 32]) in the SIMPLE algorithm. Therefore, the plasma
Figure 7. Axial distributions of electron and heavy-particle conductivity at the cathode surface is assumed to be equal to
temperatures (Te , Th , 2T-sheath model) and of the plasma roughly twice the value at the centre of the first control volume
temperature (T , LTE model) in the arc column in the vicinity of the
cathode surface; I = 40, 160 A. in the plasma, which represents a further deviation from reality.
Let us investigate this question in some detail. Let us
consider the potential difference between the first main grid
point on the arc axis, (r = 0, z = z1 ), and the centre of the
7
J. Phys. D: Appl. Phys. 45 (2012) 355201 M S Benilov et al
Table 2. Characteristics of numerical grids used: number of control volumes on the axis of the arc column and positions of the two main
grid points closest to the cathode.
Grid 1 2 3 4 5 6 7
Model 2T-sheath LTE
Number of points 40 65 80 50 55 62 70
z1 (mm) 12.022 12.020 12.008 12.100 12.060 12.035 12.022
z2 (mm) 12.070 12.062 12.025 12.300 12.181 12.106 12.065
front surface of the cathode, (r = 0, z = zw ): an average resistivity of the plasma in this interval. It is
z1 convenient to write
jz
1 w = dz. (1) Tw 1 1 1
zw = ln . (9)
1 T 1 w w
In order to evaluate integral (1) numerically, one needs
to interpolate the integrand on the interval [zw , z1 ]. A linear The lhs of this expression represents the ratio of the average
interpolation can be used for jz : resistivity of the adjacent to the cathode half of the first control
volume to the resistivity at the centre of the control volume.
z zw It is seen from table 3 that Tw /T1 and 1 /w exceed,
jz = jz(w) + jz(1) jz(w) x, x= . (2)
z1 z w respectively, 0.35 and 5 104 for all grids. It follows from
equation (9) that /1 exceeds 1500. Thus, the assumption of
However, a linear, or any algebraic, interpolation would be constant plasma conductivity in the first control volume results
inappropriate for , given its Arrhenius dependence on the in underestimating the resistance of the half-volume adjacent
plasma temperature and a strong variation of the latter in the to the cathode by a factor of more than 1500.
vicinity of the cathode surface. It seems natural to approximate The above may be summarized as follows. As seen
by an Arrhenius function of the temperature (i.e. to assume from table 3, the LTE model predicts for I = 100 A the
that ln is a linear function of 1/T in this interval) and to potential difference 1 w , i.e. the voltage drop in the
employ a linear interpolation of the temperature. The resulting adjacent to the cathode half of the first control volume, of
interpolation reads around 1 V. It is worth noting that this value does not vary
significantly between different grids, although the distance
a tw
= w exp 1 , (3) over which this potential difference occurs, z1 zw , varies
1 tw t
very considerably: from 100 to 22 m. The LTE model used
t = tw + (1 tw ) x, (4) in this work employs the assumption of plasma conductivity
being constant within a control volume, which is usual in the
where t = T /T1 , tw = Tw /T1 and a = ln (1 /w ). SIMPLE numerical algorithm. If, however, one re-evaluates
Equation (1) assumes the form the potential difference 1 w with the use of values of jz
and T from the converged LTE solution but with account of
jz(w) (z1 zw )
1 w = b, (5) variation of , then 1 w would amount not to 1 V but to
w more than 1.5 kV.
1 The procedure employed above for derivation of
ax
b= (1 + cx) exp dx, (6) equation (8) is consistent with the mathematical technique
0 tw + (1 tw ) x of evaluation of integrals of exponential functions of a large
where c = jz(1) /jz(w) 1. argument. Note that if, for example, the linear interpolation is
One can simplify equation (6) by exploiting the inequality applied to rather than to the plasma temperature, then one
w 1 . By introducing a new integration variable, which will obtain /1 = ln(1 /w ); a result incorrect by orders of
coincides with the fraction in the exponent, one obtains magnitude.
a
a + (ctw 1 + tw ) y y
b = atw e dy. (7) 5. Concluding remarks
0 [a (1 tw )y]3
The voltage over a 1 cm-long free-burning atmospheric-
Setting a , one finds that b = tw /a. [The same result
pressure argon arc, predicted by the 2T-sheath model, exhibits
may be obtained by replacing the integrand in equation (6) by
a variation with the arc current similar to the one revealed
exp (ax/tw ).] Equation (5) assumes the form
by the experiment and exceeds the experimental values by no
1 w Tw more than approximately 2 V in the current range 20175 A.
= jz(w) . (8) About two-thirds or more of the arc voltage is contributed by
z1 z w w T1 ln(1 /w )
the near-cathode sheath.
The quantity on the left-hand side (lhs) of equation (8) The model being employed describes the current transfer
represents the average electric field on the interval [zw , z1 ]. through the near-anode plasma layer in a rather crude way.
Hence, the second multiplier on the rhs may be interpreted as More accurate models [3335] indicate that the potential on
8
J. Phys. D: Appl. Phys. 45 (2012) 355201 M S Benilov et al
0 -6
2T (V) LTE
(V) -7
LTE
-8
-5
-9
grids 1 (2T), 4 (LTE) grid 4
2 (2T), 5 (LTE) 5
3 (2T), 6 (LTE) -10 6
7 (LTE) 7
-10
-11
(a) 12 14 16 18 z (mm)
20 22 (b) 12 12.2 12.4 12.6 z12.8
(mm) 13
Figure 8. Distribution of potential on the axis of the arc column calculated on different grids; I = 100 A.
Table 3. Plasma temperature, conductivity, potential and axial current density at the centre of the front surface of the cathode and at the first
and second main grid points on the arc axis obtained by means of LTE modelling on different grids; I = 100 A.
Grid 1 2 3 4
Tw (K) 3688 3660 3659 3657
T1 (K) 10 004 8915 8165 7389
T2 (K) 13 113 11901 10 933 9652
w (S m1 ) 1.03 102 8.82 103 8.77 103 8.67 103
1 (S m1 ) 2.89 103 1.80 103 1.10 103 5.20 102
2 (S m1 ) 5.94 103 4.76 103 3.82 103 2.53 103
w (V) 10.87 10.62 10.66 10.60
1 (V) 9.82 9.70 9.84 9.75
2 (V) 8.35 8.49 8.80 8.71
jz(w) (107 A m2 ) 3.12 2.85 2.60 2.13
jz(1) (107 A m2 ) 2.91 2.64 2.47 2.00
jz(2) (107 A m2 ) 2.58 2.41 2.42 2.00
the plasma side of the near-anode layer may exceed the anode employed in the LTE modelling perform this evaluation
potential by 1 or 2 V; the so-called negative anode fall. This in an inaccurate way and this inaccuracy amounts to a
may explain the above-mentioned deviation of up to about 2 V cut-off.
between the modelling and the experiment. Obviously, some cut-off or other is in place in such a
The LTE model predicts a different variation of the arc situation given the violation of the LTE in the vicinity of the
voltage with I and underestimates the experimental values cathode; at the end, switching from the arc-column equations
appreciably for low currents but by no more than approximately to the sheath equations in the 2T-sheath model also can be
2 V for I 120 A. The latter conforms to the well-known fact viewed as a kind of cut-off. The difference is that the cut-
that LTE models of high-pressure arc discharges predict arc off in numerical algorithms employed in the LTE modelling
voltages which for high currents are close to experimental
is of a numerical nature and does not reflect the physics of
values. However, the present modelling suggests that this
deviations from LTE occurring near the cathode. Therefore,
can hardly be considered as a proof of unimportance of the
the fact that this cut-off allows one to obtain arc voltages close
space-charge sheath: the LTE model overestimates both the
to experimental values for high currents but not for low currents
resistance of the bulk of the arc column and the resistance of
can hardly have physical meaning.
the part of the column that is adjacent to the cathode, and this
overestimation to a certain extent compensates for the neglect There are two-dimensional simulations of high-pressure
of the voltage drop in the near-cathode sheath. arcs disregarding the sheaths but accounting for deviations
An extremely high resistivity of the near-electrode plasma from LTE due to ambipolar diffusion (e.g. [2, 3, 36, 37])
is a known issue for LTE models of high-pressure arc and due to both ambipolar diffusion and deviation between
discharges. If the potential difference between the first main the electron and heavy-particle temperatures (e.g. [38, 39]).
grid point on the arc axis and the cathode is evaluated in terms Inclusion of diffusion currents at the electrodes overcomes
of values of jz and T taken from the LTE modelling but with a the problem of electrical conductivity at the electrodes being
due account of the dramatic variation of , which occurs in the almost zero, existing in the LTE models. An analysis of this
vicinity of the cathode, then the potential difference will be in approach in light of the results of this work is a relevant task,
excess of 1.5 kV. However, conventional numerical algorithms however, falls beyond the scope of this paper.
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J. Phys. D: Appl. Phys. 45 (2012) 355201 M S Benilov et al
10