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ARTICLES
ABSTRACT
Introduction
Measurements of long-term erosion rates are criti- 1968; Dietrich et al. 1982; Reneau et al. 1989). To
cal for understanding landform evolution, soil pro- be useful for this purpose, sedimentary deposits
duction rates, erosional effects of land use (Meyer must capture most or all of the sediment eroded
and Turner 1992), and long-term removal of atmo- from the region of interest, and must include dat-
spheric CO2 by silicate weathering (Berner et al. able stratigraphic markers (such as loess, volcanic
1983; Raymo et al. 1988). However, there have ash, or 14C-datable charcoal). Long-term denuda-
been no accurate, widely applicable methods for tion rates can also be estimated by measuring the
measuring landscape erosion rates over millennial volume of incision into an original form of known
timescales. Traditional methods for estimating age, such as a volcano (Ruxton and McDougall
catchment erosion rates rely on either measuring 1967; Seidl et al. 1994) or a marine terrace (Pillans
the present-day flux of sediment in streams, or 1988). However, datable sedimentary deposits and
measuring the volume of debris that has accumu- reconstructable forms are rare, so these methods
lated in deposits of known age. Accurately measur- for estimating erosion rates are not widely appli-
ing alluvial sediment flux is difficult, because a cable.
significant fraction of the total sediment discharge Cosmogenic nuclides have recently provided a
from a basin may occur during rare flood events new method for inferring erosion rates by revealing
(Meade 1988). Accurately estimating long-term how long mineral grains have been exposed to cos-
sediment discharge therefore requires many years mic rays near the landscape surface. Cosmogenic
of sediment flux measurements. Furthermore, nuclides record long-term erosion rates without re-
modern sediment flux measurements may be af- quiring datable deposits or surfaces, and thus pro-
fected by storage or remobilization of sediment up- vide a widely applicable technique for measuring
stream, and thus cannot be directly interpreted as erosion rates (Nishiizumi et al. 1993; Bierman
long-term erosion rates (Trimble 1977). 1994; Cerling and Craig 1994).
Denudation rates can also be estimated by mea- In situ cosmogenic nuclides are produced by sec-
suring the rate at which erosional debris has accu- ondary cosmic radiation bombarding atomic nuclei
mulated in a sedimentary deposit (e.g., Judson in minerals near the earth's surface (Lal and Peters
1967). Because the cosmic ray flux decreases expo-
Manuscript received May 31, 1995; accepted December 13,
nentially with depth below the surface, the accu-
1995. mulated cosmogenic nuclide concentration in a
2 Earth Sciences Division, Lawrence Livermore National mineral grain records the speed with which that
Laboratory, Livermore, CA 94551-9900 USA. grain has been unearthed; slower erosion rates im-
[The Journal of Geology, 1996, volume 104, p. 249-257] © 1996 by The University of Chicago. All rights reserved. 0022-1376/96/10403-0003$01.00]
249
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250 DARRYL E. GRANGER ET AL.
ply longer exposure times near the surface, and 1. Regolith Mixing, and Shielding of Underlying Bed-
thus higher concentrations. It has been shown (Lal rock. Landscapes are usually mantled by regolith,
1991) that the cosmogenic nuclide concentration which shields the underlying bedrock from cosmic
N at a steadily eroding outcrop surface is inversely radiation while at the same time subjecting indi-
proportional to the outcrop's erosion rate E, vidual sediment grains to differing cosmic ray ex-
posure histories as they are mixed by bioturbation,
soil creep, and freeze/thaw processes. What is the
N= -P (1) expected cosmogenic nuclide concentration in mo-
E
bile regolith? We consider two extreme possibili-
where Po is the nuclide production rate at the sur- ties-that the regolith is not vertically mixed, and
face and A is the absorption mean free path (the that it is vertically well-mixed-and show that
1/e attenuation length for production rate; A 60 they yield the same result. If the regolith is not
cm in rock). The nuclide concentration N averages vertically mixed, then the exhumation of individ-
the erosion rate over a time scale of order A/E, the ual grains proceeds just as with bedrock and yields
time required to erode a layer of thickness A from concentrations at the surface given by equation (1).
the surface. Equation (1) assumes that the radio- If, on the other hand, the regolith is vertically well-
active meanlife, 7, of the nuclide is much longer mixed, then the average concentration in the rego-
than A/E; for the radionuclides considered here, lith Nregoith will be the concentration inherited
26Al (T = 1.0 m.y.) and '0Be (7 = 2.2 m.y.), equation from the bedrock below (Nbedrock) plus the depth-
(1) is accurate to <6% for E > 1 cm ka-1. Because averaged nuclide production rate in the regolith
cosmogenic nuclide concentrations are insensitive (Pregolith) times the average residence time in t
to recent changes in erosion rates, they are particu- regolith (tregolith). If the regolith has thickness x,
larly useful for estimating long-term "background" average cosmogenic nuclide concentration is:
rates of erosion, as a benchmark for evaluating the
erosional effects of land use.
Nregolith ~ bedrock + Pregolith tregolith
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LONG-TERM EROSION RATES FROM NUCLIDES 251
Tournal of Geology
Equation (3) shows that cosmogenic nuclide con- fans built by these catchments. These catchments
centrations in mixed sediment can be interpreted discharge their sediments onto a basin flooded by
using equation (1) as if they were outcrop samples, Lake Lahontan during the last glacial maximum.
and that doing so yields the areally averaged ero- 14C dating of lake carbonates indicates that Lake
sion rate above the sampling location. However, Lahontan retreated from the fans' depositional area
equation (3) only holds if each of the subcatch- at 16.1 ± 0.4 ka. Lake retreat began at the top of
ments contributes sediment in proportion to its the fans' depositional area (1310 m) at 16.4 ± 0.2
long-term erosion rate. If one subcatchment con- ka and passed the bottom (1240 m) at 15.7 ± 0.1 ka
tributes a greater fraction (for example, because of (Benson 1993); 14C ages were calibrated to calendar
recent anthropogenic disturbance), then the in- ages using Bard et al. (1993). Lake Lahontan's re-
ferred catchment-average erosion rate will be bi- treat left a smooth surface of well-sorted beach
ased towards the long-term rates from that sub- sands along the shore margins below our catch-
catchment. ments. Streams discharging from the catchments
3. Storage and Remobilization of Sediment. Alluv- have deposited their sediment load as alluvial fans
ial sediment can be stored and remobilized during overlying the Lahontan beach sands (figure 1). The
its transport out of a catchment. During storage fans' volumes accurately record the long-term ero-
and transport, sediment can accumulate additional sion rates in the catchments that formed them be-
cosmogenic nuclides, or it can be shielded from cause most of the sediment is too coarse to blow
cosmic ray exposure (if it is stored at depth in allu- away by wind and there is no evidence of signifi-
vial deposits). However, the net effect on cosmo- cant chemical denudation (there is little clay, and
genic nuclide concentrations will be small as long micas and feldspars are largely unaltered).
as the mean residence time of sediment in storage We measured the fans' volumes by surveying
and transport is much shorter than the erosional their surface topography and measuring their
timescale A/E. This will be true where the total thickness at 19 widely distributed core locations,
volume of stored alluvial sediment is small com- where we drilled through the fans into the underly-
pared to the volume of sediment produced by erod- ing lake deposits, distinguishing the poorly sorted
ing the catchment by an amount A. fan sediment from the well-sorted lake sands by
This condition is met in small upland and both visual and hydrometer grain size analyses. We
mountainous catchments, where the volume of al- also surveyed the sediment contributing areas.
luvium that is stored at any time is typically small These measurements indicate that over the last
compared to A times the catchment surface area 16,000 years, catchment A has eroded at an average
(in the catchments analyzed below, it is less than rate of 5.8 ± 1.4 cm ka-1 (mean ± standard error),
15% of that volume). However, in large lowland while catchment B has eroded at 3.0 ± 0.5 cm ka- 1
river systems this may not be the case. Further- (table 1). These measurements provide an unam-
more, in large river systems that are rapidly down- biguous standard for comparison with erosion rates
cutting, and thus excavating alluvial deposits recorded by cosmogenic nuclide concentrations in
emplaced long ago, the cosmogenic nuclide con- modern-day stream sediment.
centrations in river sediment may primarily reflect We sampled stream sand that was recently dis-
the erosion rates when those deposits were em- charged from the mouths of the two catchments
placed (and radioactive decay during storage). Cos- and measured concentrations of 6Al and loBe in
mogenic nuclide methods must therefore be ap- 0.25-2 mm quartz grains from these samples (table
plied cautiously in river systems with large 2). We excluded finer grains to reduce the possibil-
volumes of stored alluvium. ity of contamination by windblown sediment from
outside the catchments. Equation (3) predicts that
each sample should record the average erosion rate
Verification of Isotopically Determined
of the upstream sediment contributing area. The
Erosion Rates
cosmogenic nuclide concentrations in sediment
To test the accuracy of the cosmogenic nuclide from the catchment mouths may therefore be di-
technique, we compared erosion rates derived from rectly compared with the catchment erosion rates
cosmogenic nuclide concentrations in alluvial sed- estimated from fan accumulation rates.
iment at two small catchments in the Fort Sage From samples A-4(a), A-4(b), A-4(c), and A-4(d),
Mountains, a granodiorite fault block in northeast we calculate that catchment A has eroded at a rate
California (figure 1) with independent long-term of E = PoA/N = 6.0 + 1.4 cm ka-l, averaged over
estimates, derived from the volumes of alluvial approximately the last A/lE 10 ka, while samples
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~ournal of Geology LONG-TERM EROSION RATES FROM NUCLIDES 253
Catchment A Catchment B
a Erosion rates (means ± standard errors) calculated from fan volumes accumulated since Lake Lahontan retreat (16.0 ± 0.4 ka),
corrected for bulk density change from bedrock (2.6 g cm-3) to fan (1.7 g cm-3). Agreement (within 1.2 standard errors) with erosion
rates inferred from cosmogenic nuclide measurements (table 2) verifies accuracy of isotope technique.
B-5(a), B-5(b), B-5(c), and B-5(d) indicate that catch- pend critically on the assumed relationships be-
ment B has eroded at 3.6 + 0.9 cm ka-l, averaged tween hillslope gradient, sediment transport rate,
over the last 17 ka (table 2). These erosion rate and erosion rate. However, there is very little em-
estimates are quantitatively consistent (within 1.2 pirical data showing what this relationship actu-
standard errors, or 1 cm ka- 1) with estimates inde-ally is. Here, using the cosmogenic nuclide tech-
pendently derived from fan accumulation since the nique verified above, we measure how erosion
retreat of Lake Lahontan. Furthermore, the two dif- rates depend on hillslope gradients in our study
ferent erosion rate estimates are averaged over catchments.
roughly the same timescale (for the cosmogenic To assess the relationship between hillslope gra-
nuclides, A/E - 10 ka at catchment A and A/E dient and erosion rates, we divided our study
17 ka at catchment B, and for fan accumulation, catchments into nine subcatchments whose aver-
approximately 16 ka). Erosion rates probably fluc- age hillslope gradients span a range from 0.2 (at the
tuated as climate changed during this time period. head of the two catchments) to 0.6 (downstream,
Since cosmogenic nuclides record an average ero- near the fault scarp). In most other respects, these
sion rate exponentially weighted towards the pres- subcatchments are quite similar; they are under-
ent, while fan accumulation averages erosion rates lain by the same bedrock, mantled with the same
linearly over time, we do not expect erosion rates regolith, covered with the same sparse vegetation,
inferred from cosmogenic nuclides to exactly and subject to the same climate. We measured
match fan accumulation. However, the generally average sideslope gradients for each subcatchment
good agreement between the two methods demon- from direct surveying. We sampled sand from the
strates quantitatively that this geochemical tech- streams where they crossed the subcatchment
nique accurately measures catchment-scale, long- boundaries and measured the concentrations of
term erosion rates under field conditions. 26A1 and 'lBe in quartz grains from each sample
(table 2). The cosmogenic nuclide concentration at
each sampling point records the average erosion
Dependence of Erosion Rates on Hillslope
rate over the entire contributing area. We calcu-
Gradient
lated the erosion rate for the area between any two
Hillslope gradient has been recognized as a critical sampling points (termed the "subcatchment ero-
factor regulating erosion rate ever since G. K. Gil- sion rate" in table 2) by correcting for the sediment
bert (1877) proposed that "erosion is most rapid flux from upstream. For example, if sampling point
where the slope is steepest." Gilbert postulated 2 lies below sampling point 1, we can calculate the
that bedrock weathers most quickly under a thin average erosion rate for the subcatchment between
soil mantle; steep hillslopes favor rapid sediment the two points, E_I, as follows:
transport, so their soil mantle is thin and their ero-
sion rates are correspondingly high. Modern land-
form evolution simulation models (e.g., Kirkby E_,A - E1A,
E_1 = 2 (4)
1971; Ahnert 1976; Willgoose et al. 1991) also de- A2 - A1
Figure 1. Oblique aerial photograph of study site, showing sediment contributing area and alluvial fan boundaries
for catchments A and B (fan thickness contours in meters). Subcatchment boundaries are shown as dashed lines.
Cosmogenic nuclide concentrations were measured in sand sampled from streams at catchment mouths and at
subcatchment boundaries.
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254 DARRYL E. GRANGER ET AL.
a Each sample was collected from modern stream sand at subcatchment boundaries indicated in figure 1. Quartz grains were
chemically isolated by a method modified from Kohl and Nishiizumi (1992).
b 26A1 and l0Be concentrations (means ± standard errors) calculated from 26A1/27Al and loBe/gBe ratios were measured by accelerator
mass spectrometry (AMS) (Davis et al. 1990), and total Al and Be concentrations were measured by flame atomic absorption
spectrophotometry (AAS).
c Erosion rates (means + standard errors) calculated from equation (1). Production rates of 26Al and 'oBe are taken as Po = 81 + 17
and 13.4 + 2.8 atoms g-'yr-', respectively, from newly revised estimates by Clark et al. (1995), scaled to 40°N latitude and 1400
m altitude (Lal 1991). (Previous estimates of production rates [Nishiizumi et al. 1989] are 20% higher.) Absorption mean free paths
of 26A1 and loBe are A = 63.9 + 3.8 and 61.2 - 3.8 cm, respectively (Nishiizumi et al. 1994) in rock of density 2.6 g cm-3
Averages are weighted by inverse variance (Bevington 1969). Uncertainties are propagated from one standard deviation AMS and
AAS measurement uncertainties; single-sample measurements are assigned an additional 15% uncertainty estimated from the
pooled intersample variability of A-4(a-d), B-2(a-c), and B-5(a-d).
Erosion rates averaged from multiple grain sizes were weighted by inverse variance and by grain size abundance in the alluvial
fans (14% <0.125 mm, 20% 0.125-0.25 mm, 24% 0.25-0.5 mm, 21% 0.5-1.0 mm, 11% 1.0-2.0 mm, and 9% >2.0 mm). In
contrast to results reported by Brown et al. (1995), there is no significant correlation between cosmogenic nuclide concentration
and grain size in samples A-4 and B-2, and only a slight negative correlation in sample B-5.
e Subcatchment erosion rates calculated from equation (4).
As figure 2 shows, erosion rates in our subcatch- at these catchments are roughly an exponential
ments vary by an order of magnitude, with the function of average hillslope gradients.
slowest erosion rates corresponding to the shallow-
est slopes, and the fastest erosion rates correspond-
discussion
ing to the steepest slopes. While our data are insuf-
ficent to describe the exact relationship between Our analysis of cosmogenic nuclide concentrations
erosion rates and hillslope gradient, and we have in stream sediment provides an important valida-
not yet accounted for other important factors such tion of a powerful new technique for inferring
as soil depth, figure 2 suggests that erosion rates catchment erosion rates. Because cosmogenic nu-
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Journal of ~eology LONG-TERM EROSION RATES FROM NUCLIDES 255
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256 DARRYL E. GRANGER ET AL.
A stream's present-day sediment load reflects re- present-day stream sediments record their ero-
cent or contemporary erosion rates, whereas the sional history, providing an accurate and widely
same sediment's cosmogenic nuclide signature re- applicable new method for measuring long-term
flects average erosion rates over millennial time- spatially averaged erosion rates.
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Tournal of Geology LONG-TERM EROSION RATES FROM NUCLIDES 257
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