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be grouped into:

emission or source characteristics the nature of the pollutant material meteorological characteristics the effects of terrain and anthropogenic structures.

Source characteristics Most industrial pollution is discharged vertically from a stack or duct into the open air. As the contaminated gas stream is emitted, the plume (body of polluted air) expands and Plume means the body of polluted air, Wind, that is horizontal air movement, will bend the plume in the downwind direction. AT some distance from the source, the plume will level off. While the plume is rising, bending, and starting to move with the wind in the downwind direction, the flue gas is being mixed and diluted by the ambient air. As the gas is being diluted by increasing volumes of air, the contaminant will eventually reach the ground. The initial rise of the plume is due to the upward inertia of the gas stream exiting the stack, and by its buoyancy. The vertical inertia is related to the exit velocity and mass of the gas. The buoyancy is related to the density relative to the surrounding air, primarily determined by temperature. Increasing exit velocity, and increasing exit temperature will increase the plume rise. The plume rise, together with the physical stack height, is called the effective stack height For a given set of stack and discharge conditions, the ground level concentration is proportional to the mass flux, i.e., the amount emitted per unit time. Increasing emission rates will therefore lead to a proportional increase in ambient concentrations. Downwind distance The greater the distance from the discharge point, the greater the volume of air available for dilution. However, since the plume starts above the ground and needs some time to reach the ground (by bending and spreading), there is no concentration observable in the immediate vicinity of the stack, then we can observe an increase for some distance as the plume approaches the ground. After this, the ground-level concentration will decrease with increasing distance from the emission source. Wind speed and direction The wind direction will determine the direction in which the plume will move across local terrain. Wind speed affects the plume rise (fast wind will bend the plume faster), and will increase the rate of dilution. Thus, the effects of wind speed work in two opposite directions:

increasing wind speed will decrease plume rise, thus increase ground level concentrations; Increasing wind speed will increase mixing, thus decreasing ground level concentrations.

Depending on the specific conditions, one or the other of these phenomena will prevail. These effects also determine the distance from the source where the maximum concentration will occur. Atmospheric stability The tendency of the atmosphere to resist or enhance vertical motion and thus turbulence is termed stability. Stability is related to both the change of temperature with height (the lapse rate) and wind speed. A neutral atmosphere neither enhances nor inhibits mechanical turbulence. An unstable atmosphere enhances turbulence, whereas a stable atmosphere inhibits mechanical turbulence. The turbulence of the atmosphere is by far the most important parameter affecting dilution of a pollutant. The more unstable the atmosphere, the greater the dilution. Stability classes are defined for different meteorological situations, characterised by wind speed and solar radiation (during the day) and cloud cover during the night. The so called Pasquill-Turner stability classes (based on D. Bruce Turners Workbook of Atmospheric Dispersion Estimates include six stability classes: 1 2 A B 3 4 5 6 Mixing height Inversions result from the vertical temperature profile of the air: while temperature normally decreases with altitude (on average, at a rate of one degree Centigrade per 100 meters), an inversions describes an increase of temperature with increasing height. This results in a stable temperature profile (the colder air is stable under the upper warmer layer), restricting vertical mixing, and exacerbating pollution episodes through restricted mixing volumes. D E F very unstable unstable C neutral stable very stable slightly unstable

Dispersion modelling A dispersion model is a mathematical description of the meteorological transport and dispersion processes, using source and meteorological parameters, for a specific period in time. The model calculations result in estimates of pollutant concentration for specific locations and times.

The mathematical models of diffusion In the current practice, two principally different types of models are applied: 1. Statistical models; 2. Dynamic models. These model types differ in their dissemination and also by the level of difficulty of their mathematical basis, their computational difficulty and the method of entry of their input parameters. Models of the first type use analytical solution based on the equation of diffusion simplified by the application of practical observation. Models of the second type are based on direct application of basic hydrodynamic and thermodynamic equations, which are solved numerically. 1. Statistical models The statistical models describe real flow in a simplified way. They are based on simplified preconditions and a set of boundary conditions: 1. The pollution source is a point with constant permanent escape of pollutants. 2. There are no spatial limiting factors. 3. The modeled case is static. 4. The diffusion of pollutants has a statistical distribution in the direction of the y and z-axis. Mathematically, the statistical models are based on the solution of the diffusion equation, where prevailing transport in the wind direction is assumed. In the vertical and horizontal direction perpendicular to the direction of the flow the turbulent diffusion is statistically described by normal distribution. 2 Dynamic models The mathematical model is formed by a system of algebraic and partial differential equations, which is solved by the method of final volumes. The definition of border conditions on the modeling area borders enables us to introduce the physical basis of the process into the model. That includes the real

characteristics of the spatial elements limiting the flow, meteorological characteristics - particularly the distribution of temperature, distribution of horizontal flow speed and so on. There are several Computer Fluid Dynamics (CFD) S/W packages available for numerical solving of the equations. These packages usually offer many options for the input of border conditions. Those can be defined as constants, functions, and eventually derivations of given quantities. The Gaussian steady-state dispersion model The most commonly used model for regulatory purposes is the so-called Gaussian steady-state model. It provides a steady-state solution to the transport and diffusion equations (transport plus diffusion = dispersion). Steady-state implies that the basic assumption is a constant emission and constant meteorological conditions: The basic Gaussian diffusion equations assumes:

that atmospheric stability and all other meteorological parameters are uniform and constant throughout the layer into which the pollutants is discharged, and in particular that wind speed and direction are uniform and constant in the domain; that turbulent diffusion is a random activity and therefor the dilution of the pollutant can be described in both horizontal and vertical directions by the Gaussian or normal distribution; that the pollutant is released at a height above the ground that is given by the physical stack height and the rise of the plume due to its momentum and buoyancy (together forming the effective stack height); that the degree of dilution is inversely proportional to the wind speed; that pollutant material reaching the ground level is reflected back into the atmosphere; that the pollutant is conservative, i.e., not undergoing any chemical reactions, transformation or decay.

The model equations The spatial dynamics of pollution dispersion is described by the following type of equation in a Gaussian model:

where

C(x, y, z) : pollutant concentration at point ( x, y, z ); U : wind speed (in the x "downwind" direction, m/s) represents the standard deviation of the concentration in the x and y direction, i.e., in the wind direction and cross-wind, in meters; Q is the emission strength (g/s) Heff is the effective stack height, see below.

From the above equation one can deduce, in steady state, the concentration in any point ( x, y, z ) in the model domain, from a constant emission rate. The effective stack height (physical stack height plus plume rise) can be computed, for example, using the formula below:

An analytical solution and a numeric solutionAnalytical solution is exact, while a numeric solution is almost always approximate. Example, solve: x = 2 analytically: x = 2 numerically: x 1.4142 You can see that very often analytic solutions involve symbols that represent numbers or equations in an exact way, while a numerical solution contains numbers that are rounded off to some degree. Atmospheric dispersion models Two fundamentally different types of atmospheric dispersion model can be identified, both based on physical dispersion equations and description of the ground surface topography: Lagrangian models and Eulerian models.

Lagrangian models Lagrangian models take different forms. The most widely used are Gaussian models. These are mechanistic models, based on turbulent eddy mixing theory, and predict for each model run a downwind ground-level concentration field of the emitted pollutant, centred on the centreline of the plume. They are primarily designed to predict short term concentration fields downwind from a source (point, line or area), but can be extended to long term average ground level concentration fields and concentration probability distributions. In the latter case, they require extensive meteorological, topographical, source location and emission time which series data. They are particularly suited for elevated point sources (e.g. power plant chimneys),

Eulerian models Eulerian dispersion models are mechanistic, based on fluid dynamics. They are designed to model high resolution concentration fields, which can be averaged to provide estimates of long term concentrations. They are particularly suited for modelling concentrations and exposures associated with complex sources, distributed over an area (e.g. road traffic). Limitations Uncertainties in dispersion models need to be recognised. These derive both from the inevitable simplification of the complex real-world processes that they entail, and from limitations of the available input data (e.g. on emission sources and meteorology). Models tend to be most reliable in relatively open, uncluttered conditions, and for estimation of longer term (daily, annual) concentrations. Because they consider only ambient concentrations, dispersion models do not provide direct estimates of human exposure. In many situations, however, ambient concentrations can be used as an indication of potential exposures and, where indoor exposures are of concern, they can be linked to indoor air pollution models.

Lagrangian and Eulerian representations In a Lagrangian coordinate system you move along with a particule about which the initial position is known. In the Lagrangian approach, the transport and diffusion are described relative to a moving coordinate system. While in Eulerian approach, the behavior of pollutant species is explained relative to a fixed coordinate system. In an Eulerian coordinate system you stand still at certain position and look at the particle when it reaches you.

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